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Sustained Water Oxidation Photocatalysis by a Bioinspired Manganese Cluster
Abstract
The generation game: A manganese–oxo complex with a cubic {Mn4O4}7+ core catalyzes the electrooxidation of water when suspended within the aqueous channels of a Nafion membrane (see picture). Illumination with visible light under an applied potential of 1.0 V (vs Ag/AgCl) generates current over one thousand turnovers. The catalytically active species arises from photolysis and subsequent dissociation of the manganese complex.
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
Water-oxidation catalysis by manganese in a geochemical-like cycle
Hocking, R. K., Brimblecombe, R., Chang, L.-Y., Singh, A., Cheah, M. H., Glover, C., Casey, W. H., & Spiccia, L. (2011) · Nature Chemistry · doi:10.1038/nchem.1049 · Cited by 517
Self-citationEfficient water oxidation at carbon nanotube–polyoxometalate electrocatalytic interfaces
Toma, F. M., Sartorel, A., Iurlo, M., Carraro, M., Parisse, P., Maccato, C., Rapino, S., Gonzalez, B. R., Amenitsch, H., Da Ros, T., et al. (2010) · Nature Chemistry · doi:10.1038/nchem.761 · Cited by 503
Metadata
- Authors
- Brimblecombe, R., Swiegers, G. F., Dismukes, G. C., & Spiccia, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2008-09-03
- Volume
- 47
- Issue
- 38
- Pages
- 7335-7338
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2142139589
- Cited by
- 295
- References
- 0
- FWCI
- 15.28
- Type
- journal article
- Language
- en
- Open access
- closed
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- Brimblecombe, R., Swiegers, G. F., Dismukes, G. C., & Spiccia, L. (2008). Sustained Water Oxidation Photocatalysis by a Bioinspired Manganese Cluster. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200801132
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