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Negative Thermal Expansion in the Metal–Organic Framework Material Cu3(1,3,5‐benzenetricarboxylate)2
Abstract
The action behind contraction: The metal–organic framework [Cu3(btc)2] displays negative thermal expansion (NTE) over a broad temperature range. This property arises from two coincident mechanisms, each of which are unique for NTE systems: the concerted transverse vibration of triangular organic linkers, and the local dynamic distortion of dinuclear metal centers within the framework lattice.
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Cited by
Evaluating metal–organic frameworks for natural gas storage
Mason, J. A., Veenstra, M., & Long, J. R. (2014) · Chem. Sci. · doi:10.1039/c3sc52633j · Cited by 1,239
Negative thermal expansion materials: technological key for control of thermal expansion
Takenaka, K. (2012) · Science and Technology of Advanced Materials · doi:10.1088/1468-6996/13/1/013001 · Cited by 586
Negative thermal expansion: a review
Miller, W., Smith, C. W., Mackenzie, D. S., & Evans, K. E. (2009) · Journal of Materials Science · doi:10.1007/s10853-009-3692-4 · Cited by 573
Coudert, F.-X. (2015) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b00046 · Cited by 528
Pronounced Negative Thermal Expansion from a Simple Structure: Cubic ScF3
Greve, B. K., Martin, K. L., Lee, P. L., Chupas, P. J., Chapman, K. W., & Wilkinson, A. P. (2010) · Journal of the American Chemical Society · doi:10.1021/ja106711v · Cited by 494
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Metadata
- Authors
- Wu, Y., Kobayashi, A., Halder, G. J., Peterson, V. K., Chapman, K. W., Lock, N., Southon, P. D., & Kepert, C. J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2008-10-28
- Volume
- 47
- Issue
- 46
- Pages
- 8929-8932
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2053225929
- Cited by
- 304
- References
- 0
- FWCI
- 6.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Negative Thermal Expansion in the Metal–Organic Framework Material Cu3(1,3,5‐benzenetricarboxylate)2. https://app.cochat.ai/papers/10.1002/anie.200803925
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- Wu, Y., Kobayashi, A., Halder, G. J., Peterson, V. K., Chapman, K. W., Lock, N., Southon, P. D., & Kepert, C. J. (2008). Negative Thermal Expansion in the Metal–Organic Framework Material Cu3(1,3,5‐benzenetricarboxylate)2. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.200803925
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