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Mechanism of Glucose Isomerization Using a Solid Lewis Acid Catalyst in Water
Abstract
Other way round: 1H and 13C NMR spectroscopy on isotopically labeled glucose reveals that in the presence of tin-containing zeolite Sn-Beta, the isomerization reaction of glucose in water proceeds by way of an intramolecular hydride shift (see scheme) rather than proton transfer. This is the first mechanistic demonstration of Sn-Beta acting as a Lewis acid in a purely aqueous environment.
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Citations
Cited by
Martínez, C., & Corma, A. (2011) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2011.03.014 · Cited by 723
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Synthesis and utilisation of sugar compounds derived from lignocellulosic biomass
Kobayashi, H., & Fukuoka, A. (2013) · Green Chemistry · doi:10.1039/c3gc00060e · Cited by 489
Activation of Carbonyl-Containing Molecules with Solid Lewis Acids in Aqueous Media
Román-Leshkov, Y., & Davis, M. E. (2011) · ACS Catalysis · doi:10.1021/cs200411d · Cited by 401
Self-citationHeterogeneous Catalysis for Tandem Reactions
Climent, M. J., Corma, A., Iborra, S., & Sabater, M. J. (2014) · ACS Catalysis · doi:10.1021/cs401052k · Cited by 361
Metadata
- Authors
- Román‐Leshkov, Y., Moliner, M., Labinger, J. A., & Davis, M. E.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2010-10-20
- Volume
- 49
- Issue
- 47
- Pages
- 8954-8957
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2096605011
- Cited by
- 725
- References
- 0
- FWCI
- 21.30
- Type
- journal article
- Language
- en
- Open access
- closed
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- Román‐Leshkov, Y., Moliner, M., Labinger, J. A., & Davis, M. E. (2010). Mechanism of Glucose Isomerization Using a Solid Lewis Acid Catalyst in Water. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201004689
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