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Structural Modifications of Mononuclear Ruthenium Complexes: A Combined Experimental and Theoretical Study on the Kinetics of Ruthenium‐Catalyzed Water Oxidation
Abstract
Small change, big difference: A minor structural modification of water-oxidation catalysts changes the kinetics of O2 evolution from second- to first-order (see scheme). According to DFT calculations, the torsional flexibility of the chelating ligands and their reorganization through the catalytic cycle are implicated in pathway selectivity, and the auxiliary carboxylate group becomes involved in proton-coupled nucleophilic attack.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Photosynthetic energy conversion: natural and artificial
Barber, J. (2009) · Chem. Soc. Rev. · doi:10.1039/b802262n · Cited by 1,843
Cited by
Artificial Photosynthesis: Molecular Systems for Catalytic Water Oxidation
Kärkäs, M. D., Verho, O., Johnston, E. V., & Åkermark, B. (2014) · Chemical Reviews · doi:10.1021/cr400572f · Cited by 1,376
Recent advances on polyoxometalate-based molecular and composite materials
Song, Y.-F., & Tsunashima, R. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35143a · Cited by 909
Efficient water oxidation catalysts based on readily available iron coordination complexes
Fillol, J. L., Codolà, Z., Garcia-Bosch, I., Gómez, L., Pla, J. J., & Costas, M. (2011) · Nature Chemistry · doi:10.1038/nchem.1140 · Cited by 784
Water oxidation catalysts based on abundant 1st row transition metals
Singh, A., & Spiccia, L. (2013) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2013.02.027 · Cited by 405
Finding the Way to Solar Fuels with Dye-Sensitized Photoelectrosynthesis Cells
Brennaman, M. K., Dillon, R. J., Alibabaei, L., Gish, M. K., Dares, C. J., Ashford, D. L., House, R. L., Meyer, G. J., Papanikolas, J. M., & Meyer, T. J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b06466 · Cited by 369
Metadata
- Authors
- Tong, L., Duan, L., Xu, Y., Privalov, T., & Sun, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2010-12-09
- Volume
- 50
- Issue
- 2
- Pages
- 445-449
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2103406080
- Cited by
- 193
- References
- 2
- FWCI
- 6.23
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tong, L., Duan, L., Xu, Y., Privalov, T., & Sun, L. (2011). Structural Modifications of Mononuclear Ruthenium Complexes: A Combined Experimental and Theoretical Study on the Kinetics of Ruthenium‐Catalyzed Water Oxidation. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201005141
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