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A Highly Efficient Photocatalytic System for Hydrogen Production by a Robust Hydrogenase Mimic in an Aqueous Solution
Abstract
A robust, inexpensive, and efficient photocatalytic system consisting of an artificial water-soluble [FeFe]-H2ase mimic 1, CdTe quantum dots, and ascorbic acid (H2A), for H2 production in pure water at room temperature has been developed. With this system, 786 μmol (17.6 mL) H2 were obtained after 10 h irradiation (λ>400 nm) with TON up to 505 and TOF up to 50 h−1 under optimized conditions.
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Cited by
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Electro- and Solar-Driven Fuel Synthesis with First Row Transition Metal Complexes
Dalle, K. E., Warnan, J., Leung, J. J., Reuillard, B., Karmel, I. S., & Reisner, E. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00392 · Cited by 912
The triplet excited state of Bodipy: formation, modulation and application
Zhao, J., Xu, K., Yang, W., Wang, Z., & Zhong, F. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00364d · Cited by 867
Robust Photogeneration of H 2 in Water Using Semiconductor Nanocrystals and a Nickel Catalyst
Han, Z., Qiu, F., Eisenberg, R., Holland, P. L., & Krauss, T. D. (2012) · Science · doi:10.1126/science.1227775 · Cited by 771
Sun, Y., Liu, C., Grauer, D. C., Yano, J., Long, J. R., Yang, P., & Chang, C. J. (2013) · Journal of the American Chemical Society · doi:10.1021/ja4094764 · Cited by 556
Metadata
- Authors
- Wang, F., Wang, W., Wang, X., Wang, H., Tung, C., & Wu, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2011-03
- Volume
- 50
- Issue
- 14
- Pages
- 3193-3197
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2002267607
- Cited by
- 348
- References
- 0
- FWCI
- 15.11
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: A Highly Efficient Photocatalytic System for Hydrogen Production by a Robust Hydrogenase Mimic in an Aqueous Solution. https://app.cochat.ai/papers/10.1002/anie.201006352
- The paper
- Wang, F., Wang, W., Wang, X., Wang, H., Tung, C., & Wu, L. (2011). A Highly Efficient Photocatalytic System for Hydrogen Production by a Robust Hydrogenase Mimic in an Aqueous Solution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201006352
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
