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Chemistry with Methane: Concepts Rather than Recipes
Abstract
Four seemingly simple transformations related to the chemistry of methane will be addressed from mechanistic and conceptual points of view: 1) metal‐mediated dehydrogenation to form metal carbene complexes, 2) the hydrogen‐atom abstraction step in the oxidative dimerization of methane, 3) the mechanisms of the CH 4→CH 3 OH conversion, and 4) the initial bond scission (CH vs. OH) as well as the rate‐limiting step in the selective CH 3 OH→CH 2 O oxidation. State‐of‐the‐art gas‐phase experiments, in conjunction with electronic‐structure calculations, permit identification of the elementary reactions at a molecular level and thus allow us to unravel detailed mechanistic aspects. Where appropriate, these results are compared with findings from related studies in solution or on surfaces.
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Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
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Carboxylate-Assisted Ruthenium-Catalyzed Alkyne Annulations by C–H/Het–H Bond Functionalizations
Ackermann, L. (2014) · Accounts of Chemical Research · doi:10.1021/ar3002798 · Cited by 1,640
Gür, T. M. (2016) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2015.10.004 · Cited by 340
The Drive to Life on Wet and Icy Worlds
Russell, M. J., Barge, L. M., Bhartia, R., Bocanegra, D., Bracher, P. J., Branscomb, E., Kidd, R., McGlynn, S., Meier, D. H., Nitschke, W., et al. (2014) · Astrobiology · doi:10.1089/ast.2013.1110 · Cited by 288
Conversion of methane to methanol on copper-containing small-pore zeolites and zeotypes
Wulfers, M. J., Teketel, S., Ipek, B., & Lobo, R. F. (2015) · Chemical Communications · doi:10.1039/c4cc09645b · Cited by 254
Metadata
- Authors
- Schwarz, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2011-06-08
- Volume
- 50
- Issue
- 43
- Pages
- 10096-10115
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2079556556
- Cited by
- 713
- References
- 1
- FWCI
- 26.07
- Type
- journal article
- Language
- en
- Open access
- closed
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