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Cryogenic Magnetocaloric Effect in a Ferromagnetic Molecular Dimer
Open accessAbstract
Molecoolers: An unprecedentedly large cryogenic magnetocaloric effect is observed in gadolinium acetate tetrahydrate (see picture, Gd pink, O red, C gray). The change in its magnetic entropy is ascribed to the high magnetic density combined with dominant ferromagnetism. For the first time in a molecular complex, direct measurements of the magnetocaloric effect corroborate indirect estimates based on heat capacity and magnetization.
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Cites
Equation of State Calculations by Fast Computing Machines
Metropolis, N., Rosenbluth, A. W., Rosenbluth, M. N., Teller, A. H., & Teller, E. (1953) · The Journal of Chemical Physics · doi:10.1063/1.1699114 · Cited by 37,192
Cited by
Molecule-based magnetic coolers
Zheng, Y.-Z., Zhou, G.-J., Zheng, Z., & Winpenny, R. E. P. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60337g · Cited by 578
High-Nuclearity 3d–4f Clusters as Enhanced Magnetic Coolers and Molecular Magnets
Peng, J.-B., Zhang, Q.-C., Kong, X.-J., Zheng, Y.-Z., Ren, Y.-P., Long, L.-S., Huang, R.-B., Zheng, L.-S., & Zheng, Z. (2012) · Journal of the American Chemical Society · doi:10.1021/ja209752z · Cited by 469
Machine learning guided design of single-molecule magnets for magnetocaloric applications
Holleis, L., Shivaram, B. S., & Balachandran, P. V. (2019) · Applied Physics Letters · doi:10.1063/1.5094553 · Cited by 29
Metadata
- Authors
- Evangelisti, M., Roubeau, O., Palacios, E., Camón, A., Hooper, T. N., Brechin, E. K., & Alonso, J. J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2011-06-07
- Volume
- 50
- Issue
- 29
- Pages
- 6606-6609
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2165523410
- Cited by
- 315
- References
- 1
- FWCI
- 14.39
- Type
- journal article
- Language
- en
- Open access
- green
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- Evangelisti, M., Roubeau, O., Palacios, E., Camón, A., Hooper, T. N., Brechin, E. K., & Alonso, J. J. (2011). Cryogenic Magnetocaloric Effect in a Ferromagnetic Molecular Dimer. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201102640
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
