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Direct Catalytic Conversion of Methane to Methanol in an Aqueous Medium by using Copper‐Promoted Fe‐ZSM‐5
Abstract
Iron copper zeolite (Fe-Cu-ZSM-5) with aqueous hydrogen peroxide is active for the selective oxidation of methane to methanol. Iron is involved in the activation of the carbon–hydrogen bond, while copper allows methanol to form as the major product. The catalyst is stable, re-usable and activates methane giving >90 % methanol selectivity and 10 % conversion in a closed catalytic cycle (see scheme).
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Citations
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Nandy, A., Zhu, J., Janet, J. P., Duan, C., Getman, R. B., & Kulik, H. J. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b02165 · Cited by 91
Metadata
- Authors
- Hammond, C., Forde, M. M., Ab Rahim, M. H., Thetford, A., He, Q., Jenkins, R. L., Dimitratos, N., Lopez‐Sanchez, J. A., Dummer, N. F., Murphy, D. M., Carley, A. F., Taylor, S. H., Willock, D. J., Stangland, E. E., Kang, J., Hagen, H., Kiely, C. J., & Hutchings, G. J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2012-04-05
- Volume
- 51
- Issue
- 21
- Pages
- 5129-5133
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2147654039
- Cited by
- 634
- References
- 0
- FWCI
- 11.71
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Hammond, C., Forde, M. M., Ab Rahim, M. H., Thetford, A., He, Q., Jenkins, R. L., Dimitratos, N., Lopez‐Sanchez, J. A., Dummer, N. F., Murphy, D. M., Carley, A. F., Taylor, S. H., Willock, D. J., Stangland, E. E., Kang, J., Hagen, H., Kiely, C. J., & Hutchings, G. J. (2012). Direct Catalytic Conversion of Methane to Methanol in an Aqueous Medium by using Copper‐Promoted Fe‐ZSM‐5. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201108706
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
