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First In Situ Observation of the LiCoO2 Electrode/Electrolyte Interface by Total‐Reflection X‐ray Absorption Spectroscopy
Abstract
Surface analysis: In situ total-reflection fluorescence X-ray absorption spectroscopy showed that reduction of cobalt at the surface of a LiCoO2 electrode occurs by contact with a liquid electrolyte. An irreversible behavior was observed at the surface of LiCoO2 during a first charge/discharge process whereas the bulk material showed a reversible behavior. This Co reduction is an initial electrode deterioration.
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Citations
Cites
Lithium Batteries: Status, Prospects and Future
Scrosati, B., & Garche, J. (2010) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.11.048 · Cited by 5,153
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An Overview on the Advances of LiCoO2 Cathodes for Lithium‐Ion Batteries
Lyu, Y., Wu, X., Wang, K., Feng, Z., Cheng, T., Liu, Y., Wang, M., Chen, R., Xu, L., Zhou, J., et al. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202000982 · Cited by 890
Non-aqueous electrolytes for sodium-ion batteries
Ponrouch, A., Monti, D., Boschin, A., Steen, B., Johansson, P., & Palacín, M. R. (2015) · Journal of Materials Chemistry A · doi:10.1039/c4ta04428b · Cited by 731
Electrode–electrolyte interfaces in lithium-based batteries
Yu, X., & Manthiram, A. (2018) · Energy & Environmental Science · doi:10.1039/c7ee02555f · Cited by 649
Zhang, J.-N., Li, Q., Wang, Y., Zheng, J., Yu, X., & Li, H. (2018) · Energy Storage Materials · doi:10.1016/j.ensm.2018.02.016 · Cited by 473
Capacitive mechanism of oxygen functional groups on carbon surface in supercapacitors
He, Y., Zhang, Y., Li, X., Lv, Z., Wang, X., Liu, Z., & Huang, X. (2018) · Electrochimica Acta · doi:10.1016/j.electacta.2018.06.103 · Cited by 355
Metadata
- Authors
- Takamatsu, D., Koyama, Y., Orikasa, Y., Mori, S., Nakatsutsumi, T., Hirano, T., Tanida, H., Arai, H., Uchimoto, Y., & Ogumi, Z.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2012-10-12
- Volume
- 51
- Issue
- 46
- Pages
- 11597-11601
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2112542398
- Cited by
- 197
- References
- 1
- FWCI
- 7.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Takamatsu, D., Koyama, Y., Orikasa, Y., Mori, S., Nakatsutsumi, T., Hirano, T., Tanida, H., Arai, H., Uchimoto, Y., & Ogumi, Z. (2012). First In Situ Observation of the LiCoO2 Electrode/Electrolyte Interface by Total‐Reflection X‐ray Absorption Spectroscopy. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201203910
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