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Magnesium Nanocrystals Embedded in a Metal–Organic Framework: Hybrid Hydrogen Storage with Synergistic Effect on Physi‐ and Chemisorption
Abstract
Hexagonal-disk-shaped magnesium nanocrystals (MgNCs) are fabricated within a porous metal-organic framework (MOF, see picture). The MgNCs@MOF stores hydrogen by both physi- and chemisorptions, exhibiting synergistic effects to decrease the isosteric heat of H(2) physisorption compared with that of pristine MOF, and decrease the H(2) chemisorption/desorption temperatures by 200 K compared with those of bare Mg powder.
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Citations
Cited by
Multifunctional metal–organic framework catalysts: synergistic catalysis and tandem reactions
Huang, Y.-B., Liang, J., Wang, X.-S., & Cao, R. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00250a · Cited by 1,908
Yu, X., Tang, Z., Sun, D., Ouyang, L., & Zhu, M. (2017) · Progress in Materials Science · doi:10.1016/j.pmatsci.2017.03.001 · Cited by 716
MOF positioning technology and device fabrication
Falcaro, P., Ricco, R., Doherty, C. M., Liang, K., Hill, A. J., & Styles, M. J. (2014) · Chem. Soc. Rev. · doi:10.1039/c4cs00089g · Cited by 710
Metal–organic framework composites and their electrochemical applications
Xue, Y., Zheng, S., Xue, H., & Pang, H. (2019) · Journal of Materials Chemistry A · doi:10.1039/c8ta12178h · Cited by 389
Empowering hydrogen storage performance of MgH2 by nanoengineering and nanocatalysis
Zhang, X. L., Liu, Y. F., Zhang, X., Hu, J. J., Gao, M. X., & Pan, H. G. (2020) · Materials Today Nano · doi:10.1016/j.mtnano.2019.100064 · Cited by 363
Metadata
- Authors
- Lim, D., Yoon, J. W., Ryu, K. Y., & Suh, M. P.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2012-09-07
- Volume
- 51
- Issue
- 39
- Pages
- 9814-9817
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2027807802
- Cited by
- 171
- References
- 0
- FWCI
- 7.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lim, D., Yoon, J. W., Ryu, K. Y., & Suh, M. P. (2012). Magnesium Nanocrystals Embedded in a Metal–Organic Framework: Hybrid Hydrogen Storage with Synergistic Effect on Physi‐ and Chemisorption. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201206055
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