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A Highly Efficient Mononuclear Iridium Complex Photocatalyst for CO2 Reduction under Visible Light
Abstract
Mononuclear iridium(III) terpyridine (tpy) 2-phenylpyridine (ppy) complexes [Ir(tpy)(R-ppy)Cl] (R=H, Me, CF3) can act as efficient and selective CO2 reduction photocatalysts. The reaction is driven using visible light in a homogeneous solution, and even in a H2O mixed solution. The most efficient photocatalyst is [Ir(tpy)(Me-ppy)Cl], for which the turnover in CO was over 50 and the quantum yield was 0.21 at 480 nm.
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Citations
Cited by
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
Molecular polypyridine-based metal complexes as catalysts for the reduction of CO2
Elgrishi, N., Chambers, M. B., Wang, X., & Fontecave, M. (2017) · Chemical Society Reviews · doi:10.1039/c5cs00391a · Cited by 555
Reaction mechanisms of catalytic photochemical CO2 reduction using Re(I) and Ru(II) complexes
Kuramochi, Y., Ishitani, O., & Ishida, H. (2018) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.11.023 · Cited by 325
Self-citationZang, Y., Li, L., Li, X., Lin, R., & Li, G. (2014) · Chemical Engineering Journal · doi:10.1016/j.cej.2014.02.068 · Cited by 289
Metadata
- Authors
- Sato, S., Morikawa, T., Kajino, T., & Ishitani, O.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2012-11-29
- Volume
- 52
- Issue
- 3
- Pages
- 988-992
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2152396877
- Cited by
- 330
- References
- 0
- FWCI
- 8.62
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sato, S., Morikawa, T., Kajino, T., & Ishitani, O. (2013). A Highly Efficient Mononuclear Iridium Complex Photocatalyst for CO2 Reduction under Visible Light. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201206137
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