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Triazine‐Based Graphitic Carbon Nitride: a Two‐Dimensional Semiconductor
Open accessAbstract
Graphitic carbon nitride has been predicted to be structurally analogous to carbon‐only graphite, yet with an inherent bandgap. We have grown, for the first time, macroscopically large crystalline thin films of triazine‐based, graphitic carbon nitride (TGCN) using an ionothermal, interfacial reaction starting with the abundant monomer dicyandiamide. The films consist of stacked, two‐dimensional (2D) crystals between a few and several hundreds of atomic layers in thickness. Scanning force and transmission electron microscopy show long‐range, in‐plane order, while optical spectroscopy, X‐ray photoelectron spectroscopy, and density functional theory calculations corroborate a direct bandgap between 1.6 and 2.0 eV. Thus TGCN is of interest for electronic devices, such as field‐effect transistors and light‐emitting diodes.
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Geim, A. K., & Novoselov, K. S. (2007) · Nature Materials · doi:10.1038/nmat1849 · Cited by 39,979
Experimental observation of the quantum Hall effect and Berry's phase in graphene
Zhang, Y., Tan, Y.-W., Stormer, H. L., & Kim, P. (2005) · Nature · doi:10.1038/nature04235 · Cited by 13,435
Two-dimensional atomic crystals
Novoselov, K. S., Jiang, D., Schedin, F., Booth, T. J., Khotkevich, V. V., Morozov, S. V., & Geim, A. K. (2005) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0502848102 · Cited by 11,788
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Electrically-Transduced Chemical Sensors Based on Two-Dimensional Nanomaterials
Meng, Z., Stolz, R. M., Mendecki, L., & Mirica, K. A. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00311 · Cited by 773
Interface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
An autonomous actuator driven by fluctuations in ambient humidity
Arazoe, H., Miyajima, D., Akaike, K., Araoka, F., Sato, E., Hikima, T., Kawamoto, M., & Aida, T. (2016) · Nature Materials · doi:10.1038/nmat4693 · Cited by 435
Metadata
- Authors
- Algara‐Siller, G., Severin, N., Chong, S. Y., Björkman, T., Palgrave, R. G., Laybourn, A., Antonietti, M., Khimyak, Y. Z., Krasheninnikov, A. V., Rabe, J. P., Kaiser, U., Cooper, A. I., Thomas, A., & Bojdys, M. J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-05-18
- Volume
- 53
- Issue
- 29
- Pages
- 7450-7455
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2170714139
- Cited by
- 670
- References
- 3
- FWCI
- 21.59
- Type
- journal article
- Language
- en
- Open access
- green
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- Algara‐Siller, G., Severin, N., Chong, S. Y., Björkman, T., Palgrave, R. G., Laybourn, A., Antonietti, M., Khimyak, Y. Z., Krasheninnikov, A. V., Rabe, J. P., Kaiser, U., Cooper, A. I., Thomas, A., & Bojdys, M. J. (2014). Triazine‐Based Graphitic Carbon Nitride: a Two‐Dimensional Semiconductor. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201402191
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