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Pd/NbOPO4 Multifunctional Catalyst for the Direct Production of Liquid Alkanes from Aldol Adducts of Furans
Abstract
Great efforts have been made to convert renewable biomass into transportation fuels. Herein, we report the novel properties of NbOx‐based catalysts in the hydrodeoxygenation of furan‐derived adducts to liquid alkanes. Excellent activity and stability were observed with almost no decrease in octane yield (>90 % throughout) in a 256 h time‐on‐stream test. Experimental and theoretical studies showed that NbOx species play the key role in CO bond cleavage. As a multifunctional catalyst, Pd/NbOPO 4 plays three roles in the conversion of aldol adducts into alkanes: 1) The noble metal (in this case Pd) is the active center for hydrogenation; 2) NbOx species help to cleave the CO bond, especially of the tetrahydrofuran ring; and 3) a niobium‐based solid acid catalyzes the dehydration, thus enabling the quantitative conversion of furan‐derived adducts into alkanes under mild conditions.
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Cited by
Selective production of arenes via direct lignin upgrading over a niobium-based catalyst
Shao, Y., Xia, Q., Dong, L., Liu, X., Han, X., Parker, S. F., Cheng, Y., Daemen, L. L., Ramirez-Cuesta, A. J., Yang, S., et al. (2017) · Nature Communications · doi:10.1038/ncomms16104 · Cited by 506
Self-citationHu, L., Lin, L., Wu, Z., Zhou, S., & Liu, S. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.02.042 · Cited by 445
Renewable bio-jet fuel production for aviation: a review
Wei, H., Liu, W., Chen, X., Yang, Q., Li, J., & Chen, H. (2019) · Fuel · doi:10.1016/j.fuel.2019.06.007 · Cited by 435
Wang, C., Zhang, X., Liu, Q., Zhang, Q., Chen, L., & Ma, L. (2020) · Fuel Processing Technology · doi:10.1016/j.fuproc.2020.106485 · Cited by 157
Highly Stable Nb2O5–Al2O3 Composites Supported Pt Catalysts for Hydrodeoxygenation of Diphenyl Ether
Guan, W., Chen, X., Jin, S., Li, C., Tsang, C.-W., & Liang, C. (2017) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.7b03736 · Cited by 67
Metadata
- Authors
- Xia, Q., Cuan, Q., Liu, X., Gong, X., Lu, G., & Wang, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-07-18
- Volume
- 53
- Issue
- 37
- Pages
- 9755-9760
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2114172214
- Cited by
- 282
- References
- 0
- FWCI
- 14.40
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Pd/NbOPO4 Multifunctional Catalyst for the Direct Production of Liquid Alkanes from Aldol Adducts of Furans. https://app.cochat.ai/papers/10.1002/anie.201403440
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- Xia, Q., Cuan, Q., Liu, X., Gong, X., Lu, G., & Wang, Y. (2014). Pd/NbOPO4 Multifunctional Catalyst for the Direct Production of Liquid Alkanes from Aldol Adducts of Furans. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201403440
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