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Catalytic Biorefining of Plant Biomass to Non‐Pyrolytic Lignin Bio‐Oil and Carbohydrates through Hydrogen Transfer Reactions
Abstract
Through catalytic hydrogen transfer reactions, a new biorefining method results in the isolation of depolymerized lignin—a non‐pyrolytic lignin bio‐oil—in addition to pulps that are amenable to enzymatic hydrolysis. Compared with organosolv lignin, the lignin bio‐oil is highly susceptible to further hydrodeoxygenation under low‐severity conditions and therefore establishes a unique platform for lignin valorization by heterogeneous catalysis. Overall, the potential of a catalytic biorefining method designed from the perspective of lignin utilization is reported.
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Cites
The Catalytic Valorization of Lignin for the Production of Renewable Chemicals
Zakzeski, J., Bruijnincx, P. C. A., Jongerius, A. L., & Weckhuysen, B. M. (2010) · Chemical Reviews · doi:10.1021/cr900354u · Cited by 4,468
Cited by
Catalytic Transformation of Lignin for the Production of Chemicals and Fuels
Li, C., Zhao, X., Wang, A., Huber, G. W., & Zhang, T. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00155 · Cited by 2,951
Guidelines for performing lignin-first biorefining
Abu-Omar, M. M., Barta, K., Beckham, G. T., Luterbacher, J. S., Ralph, J., Rinaldi, R., Román-Leshkov, Y., Samec, J. S. M., Sels, B. F., & Wang, F. (2021) · Energy & Environmental Science · doi:10.1039/d0ee02870c · Cited by 913
Self-citationAlternative Monomers Based on Lignocellulose and Their Use for Polymer Production
Delidovich, I., Hausoul, P. J. C., Deng, L., Pfützenreuter, R., Rose, M., & Palkovits, R. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00354 · Cited by 773
Wu, X., Fan, X., Xie, S., Lin, J., Cheng, J., Zhang, Q., Chen, L., & Wang, Y. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0148-8 · Cited by 649
Selective production of arenes via direct lignin upgrading over a niobium-based catalyst
Shao, Y., Xia, Q., Dong, L., Liu, X., Han, X., Parker, S. F., Cheng, Y., Daemen, L. L., Ramirez-Cuesta, A. J., Yang, S., et al. (2017) · Nature Communications · doi:10.1038/ncomms16104 · Cited by 506
Depolymerization of lignin via a non-precious Ni–Fe alloy catalyst supported on activated carbon
Zhai, Y., Li, C., Xu, G., Ma, Y., Liu, X., & Zhang, Y. (2017) · Green Chemistry · doi:10.1039/c7gc00149e · Cited by 249
Li, H., & Song, G. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b00556 · Cited by 187
Zhang, J.-W., Lu, G.-P., & Cai, C. (2017) · Green Chemistry · doi:10.1039/c7gc02087b · Cited by 101
Recent advances in hydroliquefaction of biomass for bio-oil production using in situ hydrogen donors
Zhao, B., Hu, Y., Gao, J., Zhao, G., Ray, M. B., & Xu, C. C. (2020) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.0c01649 · Cited by 56
Economical concerns of lignin in the energy sector
Sharma, A., Kaur, P., Singh, G., & Arya, S. K. (2021) · Cleaner Engineering and Technology · doi:10.1016/j.clet.2021.100258 · Cited by 38
Metadata
- Authors
- Ferrini, P., & Rinaldi, R.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-06-11
- Volume
- 53
- Issue
- 33
- Pages
- 8634-8639
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2165823311
- Cited by
- 431
- References
- 1
- FWCI
- 20.36
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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