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Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition–Sulfurization Method
Abstract
Porous films of p‐type CuInS 2, prepared by sulfurization of electrodeposited metals, are surface‐modified with thin layers of CdS and TiO 2. This specific porous electrode evolved H 2 from photoelectrochemical water reduction under simulated sunlight. Modification with thin n‐type CdS and TiO 2 layers significantly increased the cathodic photocurrent and onset potential through the formation of a p–n junction on the surface. The modified photocathodes showed a relatively high efficiency and stable H 2 production under the present reaction conditions.
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Citations
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Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Cited by
Semiconducting materials for photoelectrochemical energy conversion
Sivula, K., & van de Krol, R. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.10 · Cited by 1,645
Yang, W., Prabhakar, R. R., Tan, J., Tilley, S. D., & Moon, J. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00997j · Cited by 787
Thin-Film Materials for the Protection of Semiconducting Photoelectrodes in Solar-Fuel Generators
Hu, S., Lewis, N. S., Ager, J. W., Yang, J., McKone, J. R., & Strandwitz, N. C. (2015) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.5b05976 · Cited by 290
Metadata
- Authors
- Zhao, J., Minegishi, T., Zhang, L., Zhong, M., Gunawan, Nakabayashi, M., Ma, G., Hisatomi, T., Katayama, M., Ikeda, S., Shibata, N., Yamada, T., & Domen, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-09-10
- Volume
- 53
- Issue
- 44
- Pages
- 11808-11812
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W1976005876
- Cited by
- 203
- References
- 1
- FWCI
- 6.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, J., Minegishi, T., Zhang, L., Zhong, M., Gunawan, Nakabayashi, M., Ma, G., Hisatomi, T., Katayama, M., Ikeda, S., Shibata, N., Yamada, T., & Domen, K. (2014). Enhancement of Solar Hydrogen Evolution from Water by Surface Modification with CdS and TiO2 on Porous CuInS2 Photocathodes Prepared by an Electrodeposition–Sulfurization Method. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201406483
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