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Opposite Face Sensitivity of CeO2 in Hydrogenation and Oxidation Catalysis
Open accessAbstract
The determination of structure–performance relationships of ceria in heterogeneous reactions is enabled by the control of the crystal shape and morphology. Whereas the (100) surface, predominantly exposed in nanocubes, is optimal for CO oxidation, the (111) surface, prevalent in conventional polyhedral CeO 2 particles, dominates in C 2 H 2 hydrogenation. This result is attributed to the different oxygen vacancy chemistry on these facets. In contrast to oxidations, hydrogenations on CeO 2 are favored over low‐vacancy surfaces owing to the key role of oxygen on the stabilization of reactive intermediates. The catalytic behavior after ageing at high temperature confirms the inverse face sensitivity of the two reaction families.
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Cited by
Multi-shelled hollow micro-/nanostructures
Qi, J., Lai, X., Wang, J., Tang, H., Ren, H., Yang, Y., Jin, Q., Zhang, L., Yu, R., Ma, G., et al. (2015) · Chemical Society Reviews · doi:10.1039/c5cs00344j · Cited by 676
Zhang, S., Huang, Z.-Q., Ma, Y., Gao, W., Li, J., Cao, F., Li, L., Chang, C.-R., & Qu, Y. (2017) · Nature Communications · doi:10.1038/ncomms15266 · Cited by 508
Zaera, F. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00905 · Cited by 425
Riley, C., Zhou, S., Kunwar, D., De La Riva, A., Peterson, E., Payne, R., Gao, L., Lin, S., Guo, H., & Datye, A. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07789 · Cited by 298
An, J., Wang, Y., Lu, J., Zhang, J., Zhang, Z., Xu, S., Liu, X., Zhang, T., Gocyla, M., Heggen, M., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b01742 · Cited by 258
Metadata
- Authors
- Vilé, G., Colussi, S., Krumeich, F., Trovarelli, A., & Pérez‐Ramírez, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-08-21
- Volume
- 53
- Issue
- 45
- Pages
- 12069-12072
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2146024685
- Cited by
- 241
- References
- 0
- FWCI
- 9.23
- Type
- journal article
- Language
- en
- Open access
- green
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- Vilé, G., Colussi, S., Krumeich, F., Trovarelli, A., & Pérez‐Ramírez, J. (2014). Opposite Face Sensitivity of CeO2 in Hydrogenation and Oxidation Catalysis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201406637
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