The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Functionalization of Liquid‐Exfoliated Two‐Dimensional 2H‐MoS2
Abstract
Layered two‐dimensional (2D) inorganic transition‐metal dichalchogenides (TMDs) have attracted great interest as a result of their potential application in optoelectronics, catalysis, and medicine. However, methods to functionalize and process such 2D TMDs remain scarce. We have established a facile route towards functionalized layered MoS 2. We found that the reaction of liquid‐exfoliated 2D MoS 2, with M(OAc)2 salts (M=Ni, Cu, Zn; OAc=acetate) yielded functionalized MoS 2–M(OAc)2 materials. Importantly, this method furnished the 2H‐polytype of MoS 2 which is a semiconductor. X‐ray photoelectron spectroscopy (XPS), diffuse reflectance infrared Fourier transform spectroscopy (DRIFT–IR), and thermogravimetric analysis (TGA) provide strong evidence for the coordination of MoS 2 surface sulfur atoms to the M(OAc)2 salt. Interestingly, functionalization of 2H‐MoS 2 allows for its dispersion/processing in more conventional laboratory solvents.
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Cites
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
Self-citationThe chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Cited by
Solution‐Processed Two‐Dimensional MoS2 Nanosheets: Preparation, Hybridization, and Applications
Zhang, X., Lai, Z., Tan, C., & Zhang, H. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201509933 · Cited by 678
Samadi, M., Sarikhani, N., Zirak, M., Zhang, H., Zhang, H.-L., & Moshfegh, A. Z. (2018) · Nanoscale Horizons · doi:10.1039/c7nh00137a · Cited by 408
Scalable exfoliation and dispersion of two-dimensional materials – an update
Tao, H., Zhang, Y., Gao, Y., Sun, Z., Yan, C., & Texter, J. (2017) · Physical Chemistry Chemical Physics · doi:10.1039/c6cp06813h · Cited by 317
Intercalation and exfoliation chemistries of transition metal dichalcogenides
Zhang, Q., Mei, L., Cao, X., Tang, Y., & Zeng, Z. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta03727c · Cited by 257
Metadata
- Authors
- Backes, C., Berner, N. C., Chen, X., Lafargue, P., LaPlace, P., Freeley, M., Duesberg, G. S., Coleman, J. N., & McDonald, A. R.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-01-21
- Volume
- 54
- Issue
- 9
- Pages
- 2638-2642
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2135565097
- Cited by
- 260
- References
- 2
- FWCI
- 13.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Backes, C., Berner, N. C., Chen, X., Lafargue, P., LaPlace, P., Freeley, M., Duesberg, G. S., Coleman, J. N., & McDonald, A. R. (2015). Functionalization of Liquid‐Exfoliated Two‐Dimensional 2H‐MoS2. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201409412
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