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Frustrated Lewis Pair Chemistry: Development and Perspectives
Abstract
Frustrated Lewis pairs (FLPs) are combinations of Lewis acids and Lewis bases in solution that are deterred from strong adduct formation by steric and/or electronic factors. This opens pathways to novel cooperative reactions with added substrates. Small‐molecule binding and activation by FLPs has led to the discovery of a variety of new reactions through unprecedented pathways. Hydrogen activation and subsequent manipulation in metal‐free catalytic hydrogenations is a frequently observed feature of many FLPs. The current state of this young but rapidly expanding field is outlined in this Review and the future directions for its broadening sphere of impact are considered.
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Cited by
Synthetic Applications of Proton-Coupled Electron Transfer
Gentry, E. C., & Knowles, R. R. (2016) · Accounts of Chemical Research · doi:10.1021/acs.accounts.6b00272 · Cited by 773
Riley, C., Zhou, S., Kunwar, D., De La Riva, A., Peterson, E., Payne, R., Gao, L., Lin, S., Guo, H., & Datye, A. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b07789 · Cited by 298
Zhu, J.-B., & Chen, E. Y.-X. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08658 · Cited by 173
Wang, Q., Zhao, W., He, J., Zhang, Y., & Chen, E. Y.-X. (2017) · Macromolecules · doi:10.1021/acs.macromol.6b02398 · Cited by 127
Wang, B., Wei, Y., Li, Z., Pan, L., & Li, Y. (2018) · ChemCatChem · doi:10.1002/cctc.201801488 · Cited by 21
Metadata
- Authors
- Stephan, D. W., & Erker, G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-05-14
- Volume
- 54
- Issue
- 22
- Pages
- 6400-6441
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W1897198241
- Cited by
- 1,775
- References
- 0
- FWCI
- 96.50
- Type
- journal article
- Language
- en
- Open access
- closed
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