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Application of the Tris(acetylacetonato)iron(III)/(II) Redox Couple in p‐Type Dye‐Sensitized Solar Cells
Abstract
An electrolyte based on the tris(acetylacetonato)iron(III)/(II) redox couple ([Fe(acac)3]0/1−) was developed for p‐type dye‐sensitized solar cells (DSSCs). Introduction of a NiO blocking layer on the working electrode and the use of chenodeoxycholic acid in the electrolyte enhanced device performance by improving the photocurrent. Devices containing [Fe(acac)3]0/1− and a perylene–thiophene–triphenylamine sensitizer (PMI–6T–TPA) have the highest reported short‐circuit current (JSC=7.65 mA cm−2), and energy conversion efficiency (2.51 %) for p‐type DSSCs coupled with a fill factor of 0.51 and an open‐circuit voltage VOC=645 mV. Measurement of the kinetics of dye regeneration by the redox mediator revealed that the process is diffusion limited as the dye‐regeneration rate constant (1.7×10 8 M−1 s−1) is very close to the maximum theoretical rate constant of 3.3×10 8 M−1 s−1. Consequently, a very high dye‐regeneration yield (>99 %) could be calculated for these devices.
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Mathew, S., Yella, A., Gao, P., Humphry-Baker, R., Curchod, B. F. E., Ashari-Astani, N., Tavernelli, I., Rothlisberger, U., Nazeeruddin, M. K., & Grätzel, M. (2014) · Nature Chemistry · doi:10.1038/nchem.1861 · Cited by 4,473
Cited by
Dye-sensitized solar cells strike back
Muñoz-García, A. B., Benesperi, I., Boschloo, G., Concepcion, J. J., Delcamp, J. H., Gibson, E. A., Meyer, G. J., Pavone, M., Pettersson, H., Hagfeldt, A., et al. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01336f · Cited by 544
Mariotti, N., Bonomo, M., Fagiolari, L., Barbero, N., Gerbaldi, C., Bella, F., & Barolo, C. (2020) · Green Chemistry · doi:10.1039/d0gc01148g · Cited by 499
Finding the Way to Solar Fuels with Dye-Sensitized Photoelectrosynthesis Cells
Brennaman, M. K., Dillon, R. J., Alibabaei, L., Gish, M. K., Dares, C. J., Ashford, D. L., House, R. L., Meyer, G. J., Papanikolas, J. M., & Meyer, T. J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b06466 · Cited by 369
Liu, Q., Bottle, S. E., & Sonar, P. (2020) · Advanced Materials · doi:10.1002/adma.201903882 · Cited by 363
Metadata
- Authors
- Perera, I. R., Daeneke, T., Makuta, S., Yu, Z., Tachibana, Y., Mishra, A., Bäuerle, P., Ohlin, C. A., Bach, U., & Spiccia, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-01-28
- Volume
- 54
- Issue
- 12
- Pages
- 3758-3762
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2124512961
- Cited by
- 206
- References
- 1
- FWCI
- 11.14
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Perera, I. R., Daeneke, T., Makuta, S., Yu, Z., Tachibana, Y., Mishra, A., Bäuerle, P., Ohlin, C. A., Bach, U., & Spiccia, L. (2015). Application of the Tris(acetylacetonato)iron(III)/(II) Redox Couple in p‐Type Dye‐Sensitized Solar Cells. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201409877
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