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Radical Covalent Organic Frameworks: A General Strategy to Immobilize Open‐Accessible Polyradicals for High‐Performance Capacitive Energy Storage
Abstract
Ordered π‐columns and open nanochannels found in covalent organic frameworks (COFs) could render them able to store electric energy. However, the synthetic difficulty in achieving redox‐active skeletons has thus far restricted their potential for energy storage. A general strategy is presented for converting a conventional COF into an outstanding platform for energy storage through post‐synthetic functionalization with organic radicals. The radical frameworks with openly accessible polyradicals immobilized on the pore walls undergo rapid and reversible redox reactions, leading to capacitive energy storage with high capacitance, high‐rate kinetics, and robust cycle stability. The results suggest that channel‐wall functional engineering with redox‐active species will be a facile and versatile strategy to explore COFs for energy storage.
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Cites
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Self-citationInterface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
Porous Polymers as Multifunctional Material Platforms toward Task‐Specific Applications
Wu, J., Xu, F., Li, S., Ma, P., Zhang, X., Liu, Q., Fu, R., & Wu, D. (2019) · Advanced Materials · doi:10.1002/adma.201802922 · Cited by 555
Self-citationBeuerle, F., & Gole, B. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201710190 · Cited by 528
Metadata
- Authors
- Xu, F., Xu, H., Chen, X., Wu, D., Wu, Y., Liu, H., Gu, C., Fu, R., & Jiang, D.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-04-23
- Volume
- 54
- Issue
- 23
- Pages
- 6814-6818
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2144257491
- Cited by
- 449
- References
- 1
- FWCI
- 16.65
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xu, F., Xu, H., Chen, X., Wu, D., Wu, Y., Liu, H., Gu, C., Fu, R., & Jiang, D. (2015). Radical Covalent Organic Frameworks: A General Strategy to Immobilize Open‐Accessible Polyradicals for High‐Performance Capacitive Energy Storage. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201501706
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