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Graphitic Carbon Nitride Polymers toward Sustainable Photoredox Catalysis
Abstract
As a promising two‐dimensional conjugated polymer, graphitic carbon nitride (g‐C 3 N 4) has been utilized as a low‐cost, robust, metal‐free, and visible‐light‐active photocatalyst in the field of solar energy conversion. This Review mainly describes the latest advances in g‐C 3 N 4 photocatalysts for water splitting. Their application in CO 2 conversion, organosynthesis, and environmental purification is also briefly discussed. The methods to modify the electronic structure, nanostructure, crystal structure, and heterostructure of g‐C 3 N 4, together with correlations between its structure and performance are illustrated. Perspectives on the challenges and opportunities for the future exploration of g‐C 3 N 4 photocatalysts are provided. This Review will promote the utilization of g‐C 3 N 4 materials in the fields of photocatalysis, energy conversion, environmental remediation, and sensors.
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Cites
Electrochemical Photolysis of Water at a Semiconductor Electrode
FUJISHIMA, A., & HONDA, K. (1972) · Nature · doi:10.1038/238037a0 · Cited by 34,169
Cui, Y., Ding, Z., Liu, P., Antonietti, M., Fu, X., & Wang, X. (2012) · Phys. Chem. Chem. Phys. · doi:10.1039/c1cp22820j · Cited by 585
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Oxygen Vacancy‐Mediated Photocatalysis of BiOCl: Reactivity, Selectivity, and Perspectives
Li, H., Li, J., Ai, Z., Jia, F., & Zhang, L. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201705628 · Cited by 1,207
Hao, R., Wang, G., Tang, H., Sun, L., Xu, C., & Han, D. (2016) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2016.01.026 · Cited by 668
Selective Breaking of Hydrogen Bonds of Layered Carbon Nitride for Visible Light Photocatalysis
Kang, Y., Yang, Y., Yin, L., Kang, X., Wang, L., Liu, G., & Cheng, H. (2016) · Advanced Materials · doi:10.1002/adma.201601567 · Cited by 626
An, S., Zhang, G., Wang, T., Zhang, W., Li, K., Song, C., Miller, J. T., Miao, S., Wang, J., & Guo, X. (2018) · ACS Nano · doi:10.1021/acsnano.8b04693 · Cited by 601
Metadata
- Authors
- Zheng, Y., Lin, L., Wang, B., & Wang, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-10
- Volume
- 54
- Issue
- 44
- Pages
- 12868-12884
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2160092711
- Cited by
- 1,432
- References
- 2
- FWCI
- 51.61
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zheng, Y., Lin, L., Wang, B., & Wang, X. (2015). Graphitic Carbon Nitride Polymers toward Sustainable Photoredox Catalysis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201501788
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