The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Controlling the Structure and Length of Self‐Synthesizing Supramolecular Polymers through Nucleated Growth and Disassembly
Open accessAbstract
Directing self‐assembly processes out‐of‐equilibrium to yield kinetically trapped materials with well‐defined dimensions remains a considerable challenge. Kinetically controlled assembly of self‐synthesizing peptide‐functionalized macrocycles through a nucleation–growth mechanism is reported. Spontaneous fiber formation in this system is effectively shut down as most of the material is diverted into metastable non‐assembling trimeric and tetrameric macrocycles. However, upon adding seeds to this mixture, well‐defined fibers with controllable lengths and narrow polydispersities are obtained. This seeded growth strategy also allows access to supramolecular triblock copolymers. The resulting noncovalent assemblies can be further stabilized through covalent capture. Taken together, these results show that self‐synthesizing materials, through their interplay between dynamic covalent bonds and noncovalent interactions, are uniquely suited for out‐of‐equilibrium self‐assembly.
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Cites
Pathway Selection in Peptide Amphiphile Assembly
Korevaar, P. A., Newcomb, C. J., Meijer, E. W., & Stupp, S. I. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503882s · Cited by 265
Malakoutikhah, M., Peyralans, J. J.-P., Colomb-Delsuc, M., Fanlo-Virgós, H., Stuart, M. C. A., & Otto, S. (2013) · Journal of the American Chemical Society · doi:10.1021/ja4067805 · Cited by 111
Self-citation
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Grubbs, R. B., & Grubbs, R. H. (2017) · Macromolecules · doi:10.1021/acs.macromol.7b01440 · Cited by 396
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Sadownik, J. W., Mattia, E., Nowak, P., & Otto, S. (2016) · Nature Chemistry · doi:10.1038/nchem.2419 · Cited by 214
Self-citationLiving Supramolecular Polymerization of a Perylene Bisimide Dye into Fluorescent J‐Aggregates
Wagner, W., Wehner, M., Stepanenko, V., Ogi, S., & Würthner, F. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201709307 · Cited by 212
Metadata
- Authors
- Pal, A., Malakoutikhah, M., Leonetti, G., Tezcan, M., Colomb‐Delsuc, M., Nguyen, V. D., van der Gucht, J., & Otto, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-05-27
- Volume
- 54
- Issue
- 27
- Pages
- 7852-7856
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2152752851
- Cited by
- 165
- References
- 2
- FWCI
- 8.10
- Type
- journal article
- Language
- en
- Open access
- green
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- Pal, A., Malakoutikhah, M., Leonetti, G., Tezcan, M., Colomb‐Delsuc, M., Nguyen, V. D., van der Gucht, J., & Otto, S. (2015). Controlling the Structure and Length of Self‐Synthesizing Supramolecular Polymers through Nucleated Growth and Disassembly. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201501965
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