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In Situ Modification of Metal–Organic Frameworks in Mixed‐Matrix Membranes
Open accessAbstract
Processable films of metal–organic frameworks (MOFs) have been long sought to advance the application of MOFs in various technologies from separations to catalysis. Herein, MOF–polymer mixed‐matrix membranes (MMMs) are described, formed on several substrates using a wide variety of MOF materials. These MMMs can be delaminated from their substrates to create free‐standing MMMs that are mechanically stable and pliable. The MOFs in these MMMs remain highly crystalline, porous, and accessible for further chemical modification through postsynthetic modification (PSM) and postsynthetic exchange (PSE) processes. Overall, the findings here demonstrate a versatile approach to preparing stable functional MMMs that should contribute significantly to the advancement of these materials.
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Citations
Cited by
Metal–Organic Frameworks for Separation
Zhao, X., Wang, Y., Li, D., Bu, X., & Feng, P. (2018) · Advanced Materials · doi:10.1002/adma.201705189 · Cited by 1,305
Applications of water stable metal–organic frameworks
Wang, C., Liu, X., Keser Demir, N., Chen, J. P., & Li, K. (2016) · Chemical Society Reviews · doi:10.1039/c6cs00362a · Cited by 1,249
Metal–organic frameworks for membrane-based separations
Denny, M. S., Moreton, J. C., Benz, L., & Cohen, S. M. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2016.78 · Cited by 820
Self-citationFan, H., Gu, J., Meng, H., Knebel, A., & Caro, J. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712816 · Cited by 804
Pristine Metal–Organic Frameworks and their Composites for Energy Storage and Conversion
Liang, Z., Qu, C., Guo, W., Zou, R., & Xu, Q. (2018) · Advanced Materials · doi:10.1002/adma.201702891 · Cited by 787
Metadata
- Authors
- Denny, M. S., & Cohen, S. M.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-06-12
- Volume
- 54
- Issue
- 31
- Pages
- 9029-9032
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2163447929
- Cited by
- 449
- References
- 0
- FWCI
- 50.02
- Type
- journal article
- Language
- en
- Open access
- green
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