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Direct Imaging of Highly Anisotropic Photogenerated Charge Separations on Different Facets of a Single BiVO4 Photocatalyst
Abstract
Spatially resolved surface photovoltage spectroscopy (SRSPS) was employed to obtain direct evidence for highly anisotropic photogenerated charge separation on different facets of a single BiVO 4 photocatalyst. Through the controlled synthesis of a single crystal with preferentially exposed {010} facets, highly anisotropic photogenerated hole transfer to the {011} facet of single BiVO 4 crystals was observed. The surface photovoltage signal intensity on the {011} facet was 70 times stronger than that on the {010} facets. The influence of the built‐in electric field in the space charge region of different facets on the anisotropic photoinduced charge transfer in a single semiconductor crystal is revealed.
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Facet‐Engineered Surface and Interface Design of Photocatalytic Materials
Bai, S., Wang, L., Li, Z., & Xiong, Y. (2017) · Advanced Science · doi:10.1002/advs.201600216 · Cited by 429
Metadata
- Authors
- Zhu, J., Fan, F., Chen, R., An, H., Feng, Z., & Li, C.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-07-03
- Volume
- 54
- Issue
- 31
- Pages
- 9111-9114
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2125918160
- Cited by
- 379
- References
- 0
- FWCI
- 8.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhu, J., Fan, F., Chen, R., An, H., Feng, Z., & Li, C. (2015). Direct Imaging of Highly Anisotropic Photogenerated Charge Separations on Different Facets of a Single BiVO4 Photocatalyst. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201504135
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