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Hollow Zn/Co ZIF Particles Derived from Core–Shell ZIF‐67@ZIF‐8 as Selective Catalyst for the Semi‐Hydrogenation of Acetylene
Abstract
The rational design of metal–organic frameworks (MOFs) with hollow features and tunable porosity at the nanoscale can enhance their intrinsic properties and stimulates increasing attentions. In this Communication, we demonstrate that methanol can affect the coordination mode of ZIF‐67 in the presence of Co 2+ and induces a mild phase transformation under solvothermal conditions. By applying this transformation process to the ZIF‐67@ZIF‐8 core–shell structures, a well‐defined hollow Zn/Co ZIF rhombic dodecahedron can be obtained. The manufacturing of hollow MOFs enables us to prepare a noble metal@MOF yolk‐shell composite with controlled spatial distribution and morphology. The enhanced gas storage and porous confinement that originate from the hollow interior and coating of ZIF‐8 confers this unique catalyst with superior activity and selectivity toward the semi‐hydrogenation of acetylene.
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Citations
Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Encapsulated Metal Nanoparticles for Catalysis
Gao, C., Lyu, F., & Yin, Y. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00237 · Cited by 855
Wang, C., Kaneti, Y. V., Bando, Y., Lin, J., Liu, C., Li, J., & Yamauchi, Y. (2018) · Materials Horizons · doi:10.1039/c8mh00133b · Cited by 533
Yang, J., Zhang, F., Wang, X., He, D., Wu, G., Yang, Q., Hong, X., Wu, Y., & Li, Y. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201604315 · Cited by 380
Self-citationChen, H., Shen, K., Mao, Q., Chen, J., & Li, Y. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b03270 · Cited by 341
Self-citationZhao, S.-N., Song, X.-Z., Song, S.-Y., & Zhang, H.-J. (2017) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.02.010 · Cited by 336
Metadata
- Authors
- Yang, J., Zhang, F., Lu, H., Hong, X., Jiang, H., Wu, Y., & Li, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-08-05
- Volume
- 54
- Issue
- 37
- Pages
- 10889-10893
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2165355562
- Cited by
- 756
- References
- 1
- FWCI
- 28.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, J., Zhang, F., Lu, H., Hong, X., Jiang, H., Wu, Y., & Li, Y. (2015). Hollow Zn/Co ZIF Particles Derived from Core–Shell ZIF‐67@ZIF‐8 as Selective Catalyst for the Semi‐Hydrogenation of Acetylene. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201504242
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