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Ultrathin Free‐Standing Ternary‐Alloy Nanosheets
Abstract
A synthesis strategy for the preparation of ultrathin free‐standing ternary‐alloy nanosheets is reported. Ultrathin Pd‐Pt‐Ag nanosheets with a thickness of approximately 3 nm were successfully prepared by co‐reduction of the metal precursors in an appropriate molar ratio in the presence of CO. Both the presence of CO and the interplay between the constituent metals provide fine control over the anisotropic two‐dimensional growth of the ternary‐alloy nanostructure. The prepared Pd‐Pt‐Ag nanosheets were superior catalysts of ethanol electrooxidation owing to their specific structural and compositional characteristics. This approach will pave the way for the design of multicomponent 2D nanomaterials with unprecedented functions.
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Cites
Nanoalloys: From Theory to Applications of Alloy Clusters and Nanoparticles
Ferrando, R., Jellinek, J., & Johnston, R. L. (2008) · Chemical Reviews · doi:10.1021/cr040090g · Cited by 3,690
Highly Crystalline Multimetallic Nanoframes with Three-Dimensional Electrocatalytic Surfaces
Chen, C., Kang, Y., Huo, Z., Zhu, Z., Huang, W., Xin, H. L., Snyder, J. D., Li, D., Herron, J. A., Mavrikakis, M., et al. (2014) · Science · doi:10.1126/science.1249061 · Cited by 2,765
Freestanding palladium nanosheets with plasmonic and catalytic properties
Huang, X., Tang, S., Mu, X., Dai, Y., Chen, G., Zhou, Z., Ruan, F., Yang, Z., & Zheng, N. (2011) · Nature Nanotechnology · doi:10.1038/nnano.2010.235 · Cited by 1,602
Cited by
Metallic nanostructures with low dimensionality for electrochemical water splitting
Li, L., Wang, P., Shao, Q., & Huang, X. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00013b · Cited by 1,049
Metallenes as functional materials in electrocatalysis
Prabhu, P., & Lee, J.-M. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01041c · Cited by 427
Yang, N., Zhang, Z., Chen, B., Huang, Y., Chen, J., Lai, Z., Chen, Y., Sindoro, M., Wang, A., Cheng, H., et al. (2017) · Advanced Materials · doi:10.1002/adma.201700769 · Cited by 292
Universal strategies to multi-dimensional noble-metal-based catalysts for electrocatalysis
Gao, F., Zhang, Y., Wu, Z., You, H., & Du, Y. (2021) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.213825 · Cited by 221
Atomic Thickness Catalysts: Synthesis and Applications
Han, A., Zhang, Z., Li, X., Wang, D., & Li, Y. (2020) · Small Methods · doi:10.1002/smtd.202000248 · Cited by 43
Metadata
- Authors
- Hong, J. W., Kim, Y., Wi, D. H., Lee, S., Lee, S., Lee, Y. W., Choi, S., & Han, S. W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-01-22
- Volume
- 55
- Issue
- 8
- Pages
- 2753-2758
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2298926099
- Cited by
- 225
- References
- 3
- FWCI
- 7.24
- Type
- journal article
- Language
- en
- Open access
- closed
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