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Visible‐Light‐Driven Hydrogen Evolution Using Planarized Conjugated Polymer Photocatalysts
Open accessAbstract
Linear poly(p‐phenylene)s are modestly active UV photocatalysts for hydrogen production in the presence of a sacrificial electron donor. Introduction of planarized fluorene, carbazole, dibenzo[b,d]thiophene or dibenzo[b,d]thiophene sulfone units greatly enhances the H 2 evolution rate. The most active dibenzo[b,d]thiophene sulfone co‐polymer has a UV photocatalytic activity that rivals TiO 2, but is much more active under visible light. The dibenzo[b,d]thiophene sulfone co‐polymer has an apparent quantum yield of 2.3 % at 420 nm, as compared to 0.1 % for platinized commercial pristine carbon nitride.
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Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway
Liu, J., Liu, Y., Liu, N., Han, Y., Zhang, X., Huang, H., Lifshitz, Y., Lee, S.-T., Zhong, J., & Kang, Z. (2015) · Science · doi:10.1126/science.aaa3145 · Cited by 4,468
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Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Sulfone-containing covalent organic frameworks for photocatalytic hydrogen evolution from water
Wang, X., Chen, L., Chong, S. Y., Little, M. A., Wu, Y., Zhu, W.-H., Clowes, R., Yan, Y., Zwijnenburg, M. A., Sprick, R. S., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0141-5 · Cited by 1,320
Self-citationElectro- and Solar-Driven Fuel Synthesis with First Row Transition Metal Complexes
Dalle, K. E., Warnan, J., Leung, J. J., Reuillard, B., Karmel, I. S., & Reisner, E. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00392 · Cited by 912
Diacetylene Functionalized Covalent Organic Framework (COF) for Photocatalytic Hydrogen Generation
Pachfule, P., Acharjya, A., Roeser, J., Langenhahn, T., Schwarze, M., Schomäcker, R., Thomas, A., & Schmidt, J. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.7b11255 · Cited by 909
Benzoxazole-Linked Ultrastable Covalent Organic Frameworks for Photocatalysis
Wei, P.-F., Qi, M.-Z., Wang, Z.-P., Ding, S.-Y., Yu, W., Liu, Q., Wang, L.-K., Wang, H.-Z., An, W.-K., & Wang, W. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b00571 · Cited by 771
Metadata
- Authors
- Sprick, R. S., Bonillo, B., Clowes, R., Guiglion, P., Brownbill, N. J., Slater, B. J., Blanc, F., Zwijnenburg, M. A., Adams, D. J., & Cooper, A. I.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2015-12-22
- Volume
- 55
- Issue
- 5
- Pages
- 1792-1796
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2239682801
- Cited by
- 468
- References
- 1
- FWCI
- 11.24
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Sprick, R. S., Bonillo, B., Clowes, R., Guiglion, P., Brownbill, N. J., Slater, B. J., Blanc, F., Zwijnenburg, M. A., Adams, D. J., & Cooper, A. I. (2016). Visible‐Light‐Driven Hydrogen Evolution Using Planarized Conjugated Polymer Photocatalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201510542
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