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Extraordinary NO2 Removal by the Metal–Organic Framework UiO‐66‐NH2
Abstract
Here we discuss the removal of nitrogen dioxide, an important toxic industrial chemical and pollutant, from air using the MOF UiO‐66‐NH 2. The amine group is found to substantially aid in the removal, resulting in unprecedented removal capacities upwards of 1.4 g of NO 2 /g of MOF. Furthermore, whereas NO 2 typically generates substantial quantities of NO on sorbents, the amount generated by UiO‐66‐NH 2 is significantly reduced. Of particular significance is the formation of a diazonium ion on the aromatic ring of the MOF, and the potential reduction of NO 2 to molecular nitrogen.
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Citations
Cited by
Metal–Organic Frameworks for Separation
Zhao, X., Wang, Y., Li, D., Bu, X., & Feng, P. (2018) · Advanced Materials · doi:10.1002/adma.201705189 · Cited by 1,305
Hadjiivanov, K. I., Panayotov, D. A., Mihaylov, M. Y., Ivanova, E. Z., Chakarova, K. K., Andonova, S. M., & Drenchev, N. L. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00487 · Cited by 1,278
Metal–Organic Frameworks against Toxic Chemicals
Islamoglu, T., Chen, Z., Wasson, M. C., Buru, C. T., Kirlikovali, K. O., Afrin, U., Mian, M. R., & Farha, O. K. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00828 · Cited by 707
Sensing and capture of toxic and hazardous gases and vapors by metal–organic frameworks
Wang, H., Lustig, W. P., & Li, J. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00885f · Cited by 695
Kinetic stability of metal–organic frameworks for corrosive and coordinating gas capture
Rieth, A. J., Wright, A. M., & Dincă, M. (2019) · Nature Reviews Materials · doi:10.1038/s41578-019-0140-1 · Cited by 402
Metadata
- Authors
- Peterson, G. W., Mahle, J. J., DeCoste, J. B., Gordon, W. O., & Rossin, J. A.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-04-13
- Volume
- 55
- Issue
- 21
- Pages
- 6235-6238
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2338616383
- Cited by
- 211
- References
- 0
- FWCI
- 7.47
- Type
- journal article
- Language
- en
- Open access
- closed
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- Peterson, G. W., Mahle, J. J., DeCoste, J. B., Gordon, W. O., & Rossin, J. A. (2016). Extraordinary NO2 Removal by the Metal–Organic Framework UiO‐66‐NH2. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201601782
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