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Dry Reforming of Methane on a Highly‐Active Ni‐CeO2 Catalyst: Effects of Metal‐Support Interactions on C−H Bond Breaking
Open accessAbstract
Ni‐CeO 2 is a highly efficient, stable and non‐expensive catalyst for methane dry reforming at relative low temperatures (700 K). The active phase of the catalyst consists of small nanoparticles of nickel dispersed on partially reduced ceria. Experiments of ambient pressure XPS indicate that methane dissociates on Ni/CeO 2 at temperatures as low as 300 K, generating CHx and COx species on the surface of the catalyst. Strong metal–support interactions activate Ni for the dissociation of methane. The results of density‐functional calculations show a drop in the effective barrier for methane activation from 0.9 eV on Ni(111) to only 0.15 eV on Ni/CeO 2−x(111). At 700 K, under methane dry reforming conditions, no signals for adsorbed CHx or C species are detected in the C 1s XPS region. The reforming of methane proceeds in a clean and efficient way.
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Bruix, A., Rodriguez, J. A., Ramírez, P. J., Senanayake, S. D., Evans, J., Park, J. B., Stacchiola, D., Liu, P., Hrbek, J., & Illas, F. (2012) · Journal of the American Chemical Society · doi:10.1021/ja302070k · Cited by 839
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Cited by
A Review on Bimetallic Nickel‐Based Catalysts for CO2 Reforming of Methane
Bian, Z., Das, S., Wai, M. H., Hongmanorom, P., & Kawi, S. (2017) · ChemPhysChem · doi:10.1002/cphc.201700529 · Cited by 579
Yao, D., Yang, H., Hu, Q., Chen, Y., Chen, H., & Williams, P. T. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119413 · Cited by 258
An, J., Wang, Y., Lu, J., Zhang, J., Zhang, Z., Xu, S., Liu, X., Zhang, T., Gocyla, M., Heggen, M., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b01742 · Cited by 258
Metadata
- Authors
- Liu, Z., Grinter, D. C., Lustemberg, P. G., Nguyen‐Phan, T., Zhou, Y., Luo, S., Waluyo, I., Crumlin, E. J., Stacchiola, D. J., Zhou, J., Carrasco, J., Busnengo, H. F., Ganduglia‐Pirovano, M. V., Senanayake, S. D., & Rodriguez, J. A.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-05-04
- Volume
- 55
- Issue
- 26
- Pages
- 7455-7459
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2345834140
- Cited by
- 412
- References
- 1
- FWCI
- 9.10
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Liu, Z., Grinter, D. C., Lustemberg, P. G., Nguyen‐Phan, T., Zhou, Y., Luo, S., Waluyo, I., Crumlin, E. J., Stacchiola, D. J., Zhou, J., Carrasco, J., Busnengo, H. F., Ganduglia‐Pirovano, M. V., Senanayake, S. D., & Rodriguez, J. A. (2016). Dry Reforming of Methane on a Highly‐Active Ni‐CeO2 Catalyst: Effects of Metal‐Support Interactions on C−H Bond Breaking. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201602489
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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