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Highly Tunable Selectivity for Syngas‐Derived Alkenes over Zinc and Sodium‐Modulated Fe5C2 Catalyst
Abstract
Zn‐ and Na‐modulated Fe catalysts were fabricated by a simple coprecipitation/washing method. Zn greatly changed the size of iron species, serving as the structural promoter, while the existence of Na on the surface of the Fe catalyst alters the electronic structure, making the catalyst very active for CO activation. Most importantly, the electronic structure of the catalyst surface suppresses the hydrogenation of double bonds and promotes desorption of products, which renders the catalyst unexpectedly reactive toward alkenes—especially C 5+ alkenes (with more than 50% selectivity in hydrocarbons)—while lowering the selectivity for undesired products. This study enriches C 1 chemistry and the design of highly selective new catalysts for high‐value chemicals.
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Cites
The Fischer-Tropsch process: 1950-2000
Dry, M. E. (2002) · Catalysis Today · doi:10.1016/s0920-5861(01)00453-9 · Cited by 2,061
Cited by
Photocatalytic CO 2 conversion: What can we learn from conventional CO x hydrogenation?
Kong, T., Jiang, Y., & Xiong, Y. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00920e · Cited by 463
Zhao, Y., Waterhouse, G. I. N., Chen, G., Xiong, X., Wu, L.-Z., Tung, C.-H., & Zhang, T. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00607e · Cited by 435
Conversion of lignocellulosic biomass-derived compounds to 2-ethylhexanol: a review
Sun, C., Zhang, S., Gao, B., Yang, T., Wang, Y., Cheng, H., Zhou, H., & Chen, Z. (2024) · Environmental Chemistry Letters · doi:10.1007/s10311-024-01710-w · Cited by 16
Metadata
- Authors
- Zhai, P., Xu, C., Gao, R., Liu, X., Li, M., Li, W., Fu, X., Jia, C., Xie, J., Zhao, M., Wang, X., Li, Y., Zhang, Q., Wen, X., & Ma, D.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-07-22
- Volume
- 55
- Issue
- 34
- Pages
- 9902-9907
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2477980016
- Cited by
- 413
- References
- 1
- FWCI
- 13.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhai, P., Xu, C., Gao, R., Liu, X., Li, M., Li, W., Fu, X., Jia, C., Xie, J., Zhao, M., Wang, X., Li, Y., Zhang, Q., Wen, X., & Ma, D. (2016). Highly Tunable Selectivity for Syngas‐Derived Alkenes over Zinc and Sodium‐Modulated Fe5C2 Catalyst. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201603556
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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