The DOI matches its Crossref record; 14 of the 14 references it cites were found in a registry or an index.
Simultaneous H2 Generation and Biomass Upgrading in Water by an Efficient Noble‐Metal‐Free Bifunctional Electrocatalyst
Abstract
As an environmentally friendly approach to generate H 2, electrocatalytic water splitting has attracted worldwide interest. However, its broad employment has been inhibited by costly catalysts and low energy conversion efficiency, mainly due to the sluggish anodic half reaction, the O 2 evolution reaction (OER), whose product O 2 is not of significant value. Herein, we report an efficient strategy to replace OER with a thermodynamically more favorable reaction, the oxidation of 5‐hydroxymethylfurfural (HMF) to 2,5‐furandicarboxylic acid (FDCA), catalyzed by 3D Ni 2 P nanoparticle arrays on nickel foam (Ni 2 P NPA/NF). HMF is one of the primary dehydration intermediates of raw biomass and FDCA is of many industrial applications. As a bifunctional electrocatalyst, Ni 2 P NPA/NF is not only active for HMF oxidation but also competent for H 2 evolution. In fact, a two‐electrode electrolyzer employing Ni 2 P NPA/NF for simultaneous H 2 and FDCA production required a voltage at least 200 mV smaller compared with pure water splitting to achieve the same current density, as well as exhibiting robust stability and nearly unity Faradaic efficiencies.
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Cites
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Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
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Cited by
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Self-citationCatalytic oxidation of carbohydrates into organic acids and furan chemicals
Zhang, Z., & Huber, G. W. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00213k · Cited by 689
Pu, Z., Liu, T., Amiinu, I. S., Cheng, R., Wang, P., Zhang, C., Ji, P., Hu, W., Liu, J., & Mu, S. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202004009 · Cited by 604
Multifunctional Transition Metal‐Based Phosphides in Energy‐Related Electrocatalysis
Li, Y., Dong, Z., & Jiao, L. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902104 · Cited by 603
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Metadata
- Authors
- You, B., Jiang, N., Liu, X., & Sun, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-07-15
- Volume
- 55
- Issue
- 34
- Pages
- 9913-9917
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2470816429
- Cited by
- 615
- References
- 14
- FWCI
- 9.65
- Type
- journal article
- Language
- en
- Open access
- closed
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- You, B., Jiang, N., Liu, X., & Sun, Y. (2016). Simultaneous H2 Generation and Biomass Upgrading in Water by an Efficient Noble‐Metal‐Free Bifunctional Electrocatalyst. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201603798
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