Facile Synthesis of Three‐Dimensional Pt‐TiO 2 Nano‐networks: A Highly Active Catalyst for the Hydrolytic Dehydrogenation of Ammonia–Borane
Open accessAbstract
Three‐dimensional (3D) porous metal and metal oxide nanostructures have received considerable interest because organization of inorganic materials into 3D nanomaterials holds extraordinary properties such as low density, high porosity, and high surface area. Supramolecular self‐assembled peptide nanostructures were exploited as an organic template for catalytic 3D Pt‐TiO 2 nano‐network fabrication. A 3D peptide nanofiber aerogel was conformally coated with TiO 2 by atomic layer deposition (ALD) with angstrom‐level thickness precision. The 3D peptide‐TiO 2 nano‐network was further decorated with highly monodisperse Pt nanoparticles by using ozone‐assisted ALD. The 3D TiO 2 nano‐network decorated with Pt nanoparticles shows superior catalytic activity in hydrolysis of ammonia–borane, generating three equivalents of H 2 .
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The technological challenge of powders such as poor recoverability and reproducibility significantly restricts the industrial applicability of MOFs.
“Moreover, the technological challenge of powders such as poor recoverability and reproducibility significantly restricts the industrial applicability of MOFs.46−50”
From Bimetallic (Co/Ni) MOF-Derived CoNiP Hierarchically Porous Carbon Monolithic Aerogel for the Hydrolysis of Ammonia Borane (2024) · cites this paper as [48]
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- Authors
- Khalily, M. A., Eren, H., Akbayrak, S., Susapto, H. H., Biyikli, N., Özkar, S., & Guler, M. O.
- Affiliations
- Bilkent University (TR)
- Middle East Technical University (TR)
- Institute of Materials Science and Nanotechnology National Nanotechnology Research Center (UNAM) Bilkent University Ankara 06800 Turkey
- Department of Chemistry Middle East Technical University Ankara 06800 Turkey
- Corresponding author
- Guler, Mustafa O.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2016-09-06
- Volume
- 55
- Issue
- 40
- Pages
- 12257-12261
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2511519823
- Cited by
- 181
- References
- 36
- Citations by year
- 2026: 8 · 2025: 12 · 2024: 11 · 2023: 17 · 2022: 15 · 2021: 22 · 2020: 21 · 2019: 25 · 2018: 23 · 2017: 25 · 2016: 2
- FWCI
- 11.14
- Type
- journal article
- Language
- en
- Open access
- green
- hdl.handle.net
- Licence
- Locations
- Angewandte Chemie International Edition (publishedVersion)
- PubMed (publishedVersion)
- Bilkent University Institutional Repository (Bilkent University) (submittedVersion)
- OpenMETU (Middle East Technical University) (submittedVersion, cc-by-nc-nd)
- Funders
- TUBITAK (112M578)
- Turkish Academy of Sciences
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
- Physical Sciences › Chemistry › Inorganic Chemistry › Metal-Organic Frameworks: Synthesis and Applications
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › TiO2 Photocatalysis and Solar Cells
- Keywords
- three-dimensional nanostructures, ammonia borane hydrolysis, dehydrogenation, hydrogen storage, peptide nanofibers, atomic layer deposition, platinum nanoparticles, supramolecular self-assembly, metal oxide nanostructures
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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