The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Robust Binding between Carbon Nitride Nanosheets and a Binuclear Ruthenium(II) Complex Enabling Durable, Selective CO2 Reduction under Visible Light in Aqueous Solution
Abstract
Carbon nitride nanosheets (NS‐C 3 N 4) were found to undergo robust binding with a binuclear ruthenium(II) complex (RuRu′) even in basic aqueous solution. A hybrid material consisting of NS‐C 3 N 4 (further modified with nanoparticulate Ag) and RuRu′ promoted the photocatalytic reduction of CO 2 to formate in aqueous media, in conjunction with high selectivity (approximately 98 %) and a good turnover number (>2000 with respect to the loaded Ru complex). These represent the highest values yet reported for a powder‐based photocatalytic system during CO 2 reduction under visible light in an aqueous environment. We also assessed the desorption of RuRu′ from the Ag/C 3 N 4 surface, a factor that can contribute to a loss of activity. It was determined that desorption is not induced by salt additives, pH changes, or photoirradiation, which partly explains the high photocatalytic performance of this material.
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Citations
Cites
Photocatalytic Water Splitting: Recent Progress and Future Challenges
Maeda, K., & Domen, K. (2010) · The Journal of Physical Chemistry Letters · doi:10.1021/jz1007966 · Cited by 2,739
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Cited by
Zhao, Y., Waterhouse, G. I. N., Chen, G., Xiong, X., Wu, L.-Z., Tung, C.-H., & Zhang, T. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00607e · Cited by 435
Xia, P., Antonietti, M., Zhu, B., Heil, T., Yu, J., & Cao, S. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201900093 · Cited by 367
Reaction mechanisms of catalytic photochemical CO2 reduction using Re(I) and Ru(II) complexes
Kuramochi, Y., Ishitani, O., & Ishida, H. (2018) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2017.11.023 · Cited by 325
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Metadata
- Authors
- Kuriki, R., Yamamoto, M., Higuchi, K., Yamamoto, Y., Akatsuka, M., Lu, D., Yagi, S., Yoshida, T., Ishitani, O., & Maeda, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-04-07
- Volume
- 56
- Issue
- 17
- Pages
- 4867-4871
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2604629119
- Cited by
- 258
- References
- 1
- FWCI
- 11.46
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Kuriki, R., Yamamoto, M., Higuchi, K., Yamamoto, Y., Akatsuka, M., Lu, D., Yagi, S., Yoshida, T., Ishitani, O., & Maeda, K. (2017). Robust Binding between Carbon Nitride Nanosheets and a Binuclear Ruthenium(II) Complex Enabling Durable, Selective CO2 Reduction under Visible Light in Aqueous Solution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201701627
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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