The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Self‐Optimization of the Active Site of Molybdenum Disulfide by an Irreversible Phase Transition during Photocatalytic Hydrogen Evolution
Abstract
The metallic 1T‐MoS 2 has attracted considerable attention as an effective catalyst for hydrogen evolution reactions (HERs). However, the fundamental mechanism about the catalytic activity of 1T‐MoS 2 and the associated phase evolution remain elusive and controversial. Herein, we prepared the most stable 1T‐MoS 2 by hydrothermal exfoliation of MoS 2 nanosheets vertically rooted into rigid one‐dimensional TiO 2 nanofibers. The 1T‐MoS 2 can keep highly stable over one year, presenting an ideal model system for investigating the HER catalytic activities as a function of the phase evolution. Both experimental studies and theoretical calculations suggest that 1T phase can be irreversibly transformed into a more active 1T′ phase as true active sites in photocatalytic HERs, resulting in a “catalytic site self‐optimization”. Hydrogen atom adsorption is the major driving force for this phase transition.
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Cites
MoS 2 Nanoparticles Grown on Graphene: An Advanced Catalyst for the Hydrogen Evolution Reaction
Li, Y., Wang, H., Xie, L., Liang, Y., Hong, G., & Dai, H. (2011) · Journal of the American Chemical Society · doi:10.1021/ja201269b · Cited by 5,001
Lu, Q., Yu, Y., Ma, Q., Chen, B., & Zhang, H. (2016) · Advanced Materials · doi:10.1002/adma.201503270 · Cited by 1,447
Zhou, W., Yin, Z., Du, Y., Huang, X., Zeng, Z., Fan, Z., Liu, H., Wang, J., & Zhang, H. (2013) · Small · doi:10.1002/smll.201201161 · Cited by 1,258
Solution‐Processed Two‐Dimensional MoS2 Nanosheets: Preparation, Hybridization, and Applications
Zhang, X., Lai, Z., Tan, C., & Zhang, H. (2016) · Angewandte Chemie International Edition · doi:10.1002/anie.201509933 · Cited by 678
Cited by
Roadmap and Direction toward High-Performance MoS 2 Hydrogen Evolution Catalysts
Cao, Y. (2021) · ACS Nano · doi:10.1021/acsnano.1c01879 · Cited by 405
Zhang, S., Zhang, Z., Si, Y., Li, B., Deng, F., Yang, L., Liu, X., Dai, W., & Luo, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c05834 · Cited by 394
Self-citationSynthesis, stabilization and applications of 2-dimensional 1T metallic MoS 2
Shi, S., Sun, Z., & Hu, Y. H. (2018) · Journal of Materials Chemistry A · doi:10.1039/c8ta08152b · Cited by 374
Wang, J., Fang, W., Hu, Y., Zhang, Y., Dang, J., Wu, Y., Chen, B., Zhao, H., & Li, Z. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2021.120490 · Cited by 259
Liu, J., Xu, H., Yan, J., Huang, J., Song, Y., Deng, J., Wu, J., Ding, C., Wu, X., Yuan, S., et al. (2019) · Journal of Materials Chemistry A · doi:10.1039/c9ta05399a · Cited by 50
Metadata
- Authors
- Wang, L., Liu, X., Luo, J., Duan, X., Crittenden, J., Liu, C., Zhang, S., Pei, Y., Zeng, Y., & Duan, X.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-05-23
- Volume
- 56
- Issue
- 26
- Pages
- 7610-7614
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2784545720
- Cited by
- 262
- References
- 4
- FWCI
- 9.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, L., Liu, X., Luo, J., Duan, X., Crittenden, J., Liu, C., Zhang, S., Pei, Y., Zeng, Y., & Duan, X. (2017). Self‐Optimization of the Active Site of Molybdenum Disulfide by an Irreversible Phase Transition during Photocatalytic Hydrogen Evolution. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201703066
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