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Full Selectivity Control in Cobalt(III)‐Catalyzed C−H Alkylations by Switching of the C−H Activation Mechanism
Abstract
Selectivity control in hydroarylation‐based C−H alkylation has been dominated by steric interactions. A conceptually distinct strategy that exploits the programmed switch in the C−H activation mechanism by means of cobalt catalysis is presented, which sets the stage for convenient C−H alkylations with unactivated alkenes. Detailed mechanistic studies provide compelling evidence for a programmable switch in the C−H activation mechanism from a linear‐selective ligand‐to‐ligand hydrogen transfer to a branched‐selective base‐assisted internal electrophilic‐type substitution.
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Cites
Effect of the damping function in dispersion corrected density functional theory
Grimme, S., Ehrlich, S., & Goerigk, L. (2011) · Journal of Computational Chemistry · doi:10.1002/jcc.21759 · Cited by 28,221
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3d Transition Metals for C–H Activation
Gandeepan, P., Müller, T., Zell, D., Cera, G., Warratz, S., & Ackermann, L. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00507 · Cited by 2,332
Self-citationMetal-catalyzed regiodivergent organic reactions
Nájera, C., Beletskaya, I. P., & Yus, M. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00872h · Cited by 304
Metadata
- Authors
- Zell, D., Bursch, M., Müller, V., Grimme, S., & Ackermann, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-07-24
- Volume
- 56
- Issue
- 35
- Pages
- 10378-10382
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2635391339
- Cited by
- 277
- References
- 1
- FWCI
- 17.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Full Selectivity Control in Cobalt(III)‐Catalyzed C−H Alkylations by Switching of the C−H Activation Mechanism. https://app.cochat.ai/papers/10.1002/anie.201704196
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- Zell, D., Bursch, M., Müller, V., Grimme, S., & Ackermann, L. (2017). Full Selectivity Control in Cobalt(III)‐Catalyzed C−H Alkylations by Switching of the C−H Activation Mechanism. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201704196
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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
