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para‐Xylene Ultra‐selective Zeolite MFI Membranes Fabricated from Nanosheet Monolayers at the Air–Water Interface
Open accessAbstract
The control of membrane morphology and microstructure is crucial to improve the separation performance of molecular‐sieve membranes. This can be enabled by making thin, dense, and uniform seed‐crystal coatings, which are then intergrown into continuous membranes. Herein, we show a novel and simple floating particle coating method can give closely packed monolayers of zeolite nanosheets on nonporous or porous supports. The zeolite nanosheet monolayer is formed at the air–water interface in a conical Teflon trough. As the water in the trough is drained, the monolayer is deposited on a support placed below. Membranes prepared by gel‐free secondary growth of the nanosheets deposited by this method show unprecedented ultra‐selective performance for separation of para‐ from ortho‐xylene (separation factor >10 000).
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Cites
Ordered porous materials for emerging applications
Davis, M. E. (2002) · Nature · doi:10.1038/nature00785 · Cited by 5,308
Seven chemical separations to change the world
Sholl, D. S., & Lively, R. P. (2016) · Nature · doi:10.1038/532435a · Cited by 4,769
Cited by
Emerging applications of zeolites in catalysis, separation and host–guest assembly
Li, Y., & Yu, J. (2021) · Nature Reviews Materials · doi:10.1038/s41578-021-00347-3 · Cited by 585
Nonporous Adaptive Crystals of Pillararenes
Jie, K., Zhou, Y., Li, E., & Huang, F. (2018) · Accounts of Chemical Research · doi:10.1021/acs.accounts.8b00255 · Cited by 533
Microporous framework membranes for precise molecule/ion separations
Dou, H., Xu, M., Wang, B., Zhang, Z., Wen, G., Zheng, Y., Luo, D., Zhao, L., Yu, A., Zhang, L., et al. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00552e · Cited by 371
Near-Ideal Xylene Selectivity in Adaptive Molecular Pillar[n]arene Crystals
Jie, K., Liu, M., Zhou, Y., Little, M. A., Pulido, A., Chong, S. Y., Stephenson, A., Hughes, A. R., Sakakibara, F., Ogoshi, T., et al. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b02621 · Cited by 258
Metadata
- Authors
- Kim, D., Jeon, M. Y., Stottrup, B. L., & Tsapatsis, M.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-12-11
- Volume
- 57
- Issue
- 2
- Pages
- 480-485
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2774093975
- Cited by
- 164
- References
- 2
- FWCI
- 14.14
- Type
- journal article
- Language
- en
- Open access
- green
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- Kim, D., Jeon, M. Y., Stottrup, B. L., & Tsapatsis, M. (2018). para‐Xylene Ultra‐selective Zeolite MFI Membranes Fabricated from Nanosheet Monolayers at the Air–Water Interface. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201708835
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