The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Van der Waals Heterostructures Comprised of Ultrathin Polymer Nanosheets for Efficient Z‐Scheme Overall Water Splitting
Abstract
Inspired by natural photosynthesis, Z‐scheme photocatalytic systems are very appealing for achieving efficient overall water splitting. Developing metal‐free Z‐scheme photocatalysts for overall water splitting, however, still remains challenging. The construction of polymer‐based van der Waals heterostructures as metal‐free Z‐scheme photocatalytic systems for overall water splitting is described using aza‐fused microporous polymers (CMP) and C 2 N ultrathin nanosheets as O 2‐ and H 2‐evolving catalysts, respectively. Although neither polymer is able to split pure water using visible light, a 2:1 stoichiometric ratio of H 2 and O 2 was observed when aza‐CMP/C 2 N heterostructures were used. A solar‐to‐hydrogen conversion efficiency of 0.23 % was determined, which could be further enhanced to 0.40 % by using graphene as the solid electron mediator to promote the interfacial charge‐transfer process. This study highlights the potential of polymer photocatalysts for overall water splitting.
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Cites
Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
An efficient and pH-universal ruthenium-based catalyst for the hydrogen evolution reaction
Mahmood, J., Li, F., Jung, S.-M., Okyay, M. S., Ahmad, I., Kim, S.-J., Park, N., Jeong, H. Y., & Baek, J.-B. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2016.304 · Cited by 1,685
Wang, Q., Hisatomi, T., Jia, Q., Tokudome, H., Zhong, M., Wang, C., Pan, Z., Takata, T., Nakabayashi, M., Shibata, N., et al. (2016) · Nature Materials · doi:10.1038/nmat4589 · Cited by 1,684
Meng, F., Li, J., Cushing, S. K., Zhi, M., & Wu, N. (2013) · Journal of the American Chemical Society · doi:10.1021/ja404851s · Cited by 643
Cited by
Zhao, D., Wang, Y., Dong, C.-L., Huang, Y.-C., Chen, J., Xue, F., Shen, S., & Guo, L. (2021) · Nature Energy · doi:10.1038/s41560-021-00795-9 · Cited by 1,379
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Jing, J., Yang, J., Li, W., Wu, Z., & Zhu, Y. (2022) · Advanced Materials · doi:10.1002/adma.202106807 · Cited by 367
Wan, Y., Wang, L., Xu, H., Wu, X., & Yang, J. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00564 · Cited by 363
Self-citationEngineering β-ketoamine covalent organic frameworks for photocatalytic overall water splitting
Yang, Y., Chu, X., Zhang, H.-Y., Zhang, R., Liu, Y.-H., Zhang, F.-M., Lu, M., Yang, Z.-D., & Lan, Y.-Q. (2023) · Nature Communications · doi:10.1038/s41467-023-36338-x · Cited by 281
Metadata
- Authors
- Wang, L., Zheng, X., Chen, L., Xiong, Y., & Xu, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-02-22
- Volume
- 57
- Issue
- 13
- Pages
- 3454-3458
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2791723510
- Cited by
- 329
- References
- 4
- FWCI
- 9.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, L., Zheng, X., Chen, L., Xiong, Y., & Xu, H. (2018). Van der Waals Heterostructures Comprised of Ultrathin Polymer Nanosheets for Efficient Z‐Scheme Overall Water Splitting. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201710557
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