The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Integration of Plasmonic Effects and Schottky Junctions into Metal–Organic Framework Composites: Steering Charge Flow for Enhanced Visible‐Light Photocatalysis
Abstract
A wide range of light absorption and rapid electron–hole separation are desired for efficient photocatalysis. Herein, on the basis of a semiconductor‐like metal–organic framework (MOF), a Pt@MOF/Au catalyst with two types of metal–MOF interfaces integrates the surface plasmon resonance excitation of Au nanorods with a Pt‐MOF Schottky junction, which not only extends the light absorption of the MOF from the UV to the visible region but also greatly accelerates charge transfer. The spatial separation of Pt and Au particles by the MOF further steers the formation of charge flow and expedites the charge migration. As a result, the Pt@MOF/Au presents an exceptionally high photocatalytic H 2 production rate by water splitting under visible light irradiation, far superior to Pt/MOF/Au, MOF/Au and other counterparts with similar Pt or Au contents, highlighting the important role of each component and the Pt location in the catalyst.
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Citations
Cites
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
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Cited by
Bavykina, A., Kolobov, N., Khan, I. S., Bau, J. A., Ramirez, A., & Gascon, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00685 · Cited by 1,754
Metal–organic frameworks as a platform for clean energy applications
Li, X., Yang, X., Xue, H., Pang, H., & Xu, Q. (2020) · EnergyChem · doi:10.1016/j.enchem.2020.100027 · Cited by 706
Metal–Organic Frameworks as Photocatalysts for Solar-Driven Overall Water Splitting
Navalón, S., Dhakshinamoorthy, A., Álvaro, M., Ferrer, B., & García, H. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00460 · Cited by 538
Li, G., Zhao, S., Zhang, Y., & Tang, Z. (2018) · Advanced Materials · doi:10.1002/adma.201800702 · Cited by 521
Jin, P., Wang, L., Ma, X., Lian, R., Huang, J., She, H., Zhang, M., & Wang, Q. (2021) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.119762 · Cited by 339
Metadata
- Authors
- Xiao, J., Han, L., Luo, J., Yu, S., & Jiang, H.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2017-12-21
- Volume
- 57
- Issue
- 4
- Pages
- 1103-1107
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2772342945
- Cited by
- 569
- References
- 1
- FWCI
- 12.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xiao, J., Han, L., Luo, J., Yu, S., & Jiang, H. (2018). Integration of Plasmonic Effects and Schottky Junctions into Metal–Organic Framework Composites: Steering Charge Flow for Enhanced Visible‐Light Photocatalysis. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201711725
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