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A Permselective CeOx Coating To Improve the Stability of Oxygen Evolution Electrocatalysts
Abstract
Highly active NiFeOx electrocatalysts for the oxygen evolution reaction (OER) suffer gradual deactivation with time owing to the loss of Fe species from the active sites into solution during catalysis. The anodic deposition of a CeOx layer prevents the loss of such Fe species from the OER catalysts, achieving a highly stable performance. The CeOx layer does not affect the OER activity of the catalyst underneath but exhibits unique permselectivity, allowing the permeation of OH− and O 2 through while preventing the diffusion of redox ions through the layer to function as a selective O 2‐evolving electrode. The use of such a permselective protective layer provides a new strategy for improving the durability of electrocatalysts.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
Luo, J., Im, J.-H., Mayer, M. T., Schreier, M., Nazeeruddin, M. K., Park, N.-G., Tilley, S. D., Fan, H. J., & Grätzel, M. (2014) · Science · doi:10.1126/science.1258307 · Cited by 2,509
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Tong, W., Forster, M., Dionigi, F., Dresp, S., Sadeghi Erami, R., Strasser, P., Cowan, A. J., & Farràs, P. (2020) · Nature Energy · doi:10.1038/s41560-020-0550-8 · Cited by 1,299
Fe-Based Electrocatalysts for Oxygen Evolution Reaction: Progress and Perspectives
Feng, C., Faheem, M. B., Fu, J., Xiao, Y., Li, C., & Li, Y. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b05445 · Cited by 587
Stability of electrocatalytic OER: from principle to application
Li, H., Lin, Y., Duan, J., Wen, Q., Liu, Y., & Zhai, T. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00010a · Cited by 540
Water Electrolysis toward Elevated Temperature: Advances, Challenges and Frontiers
Zhang, W., Liu, M., Gu, X., Shi, Y., Deng, Z., & Cai, N. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00573 · Cited by 441
Emerging materials and technologies for electrocatalytic seawater splitting
Jin, H., Xu, J., Liu, H., Shen, H., Yu, H., Jaroniec, M., Zheng, Y., & Qiao, S.-Z. (2023) · Science Advances · doi:10.1126/sciadv.adi7755 · Cited by 417
Metadata
- Authors
- Obata, K., & Takanabe, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-01-05
- Volume
- 57
- Issue
- 6
- Pages
- 1616-1620
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2773713171
- Cited by
- 213
- References
- 2
- FWCI
- 2.49
- Type
- journal article
- Language
- en
- Open access
- closed
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- Obata, K., & Takanabe, K. (2018). A Permselective CeOx Coating To Improve the Stability of Oxygen Evolution Electrocatalysts. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201712121
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