The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Promoted Fixation of Molecular Nitrogen with Surface Oxygen Vacancies on Plasmon‐Enhanced TiO2 Photoelectrodes
Abstract
A hundred years on, the energy‐intensive Haber–Bosch process continues to turn the N 2 in air into fertilizer, nourishing billions of people while causing pollution and greenhouse gas emissions. The urgency of mitigating climate change motivates society to progress toward a more sustainable method for fixing N 2 that is based on clean energy. Surface oxygen vacancies (surface O vac) hold great potential for N 2 adsorption and activation, but introducing O vac on the very surface without affecting bulk properties remains a great challenge. Fine tuning of the surface O vac by atomic layer deposition is described, forming a thin amorphous TiO 2 layer on plasmon‐enhanced rutile TiO 2/Au nanorods. Surface O vac in the outer amorphous TiO 2 thin layer promote the adsorption and activation of N 2, which facilitates N 2 reduction to ammonia by excited electrons from ultraviolet‐light‐driven TiO 2 and visible‐light‐driven Au surface plasmons. The findings offer a new approach to N 2 photofixation under ambient conditions (that is, room temperature and atmospheric pressure).
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Cites
Chemistry and Properties of Nanocrystals of Different Shapes
Burda, C., Chen, X., Narayanan, R., & El-Sayed, M. A. (2005) · Chemical Reviews · doi:10.1021/cr030063a · Cited by 7,230
Cited by
Yang, J., Guo, Y., Jiang, R., Qin, F., Zhang, H., Lu, W., Wang, J., & Yu, J. C. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.8b03537 · Cited by 499
Oxygen vacancies in metal oxides: recent progress towards advanced catalyst design
Zhuang, G., Chen, Y., Zhuang, Z., Yu, Y., & Yu, J. (2020) · Science China Materials · doi:10.1007/s40843-020-1305-6 · Cited by 499
Kumar, A., Choudhary, P., Kumar, A., Camargo, P. H. C., & Krishnan, V. (2022) · Small · doi:10.1002/smll.202101638 · Cited by 441
Li, B., Lai, C., Zeng, G., Huang, D., Qin, L., Zhang, M., Cheng, M., Liu, X., Yi, H., Zhou, C., et al. (2019) · Small · doi:10.1002/smll.201804565 · Cited by 367
Han, J., Liu, Z., Ma, Y., Cui, G., Xie, F., Wang, F., Wu, Y., Gao, S., Xu, Y., & Sun, X. (2018) · Nano Energy · doi:10.1016/j.nanoen.2018.07.045 · Cited by 361
Metadata
- Authors
- Li, C., Wang, T., Zhao, Z., Yang, W., Li, J., Li, A., Yang, Z., Ozin, G. A., & Gong, J.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-03-08
- Volume
- 57
- Issue
- 19
- Pages
- 5278-5282
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2793865460
- Cited by
- 454
- References
- 1
- FWCI
- 14.42
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, C., Wang, T., Zhao, Z., Yang, W., Li, J., Li, A., Yang, Z., Ozin, G. A., & Gong, J. (2018). Promoted Fixation of Molecular Nitrogen with Surface Oxygen Vacancies on Plasmon‐Enhanced TiO2 Photoelectrodes. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201713229
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