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Highly Stable Aqueous Zinc‐Ion Storage Using a Layered Calcium Vanadium Oxide Bronze Cathode
Abstract
Cost‐effective aqueous rechargeable batteries are attractive alternatives to non‐aqueous cells for stationary grid energy storage. Among different aqueous cells, zinc‐ion batteries (ZIBs), based on Zn 2+ intercalation chemistry, stand out as they can employ high‐capacity Zn metal as the anode material. Herein, we report a layered calcium vanadium oxide bronze as the cathode material for aqueous Zn batteries. For the storage of the Zn 2+ ions in the aqueous electrolyte, we demonstrate that the calcium‐based bronze structure can deliver a high capacity of 340 mA h g−1 at 0.2 C, good rate capability, and very long cycling life (96 % retention after 3000 cycles at 80 C). Further, we investigate the Zn 2+ storage mechanism, and the corresponding electrochemical kinetics in this bronze cathode. Finally, we show that our Zn cell delivers an energy density of 267 W h kg−1 at a power density of 53.4 W kg−1.
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Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Rechargeable Batteries for Grid Scale Energy Storage
Zhu, Z., Jiang, T., Ali, M., Meng, Y., Jin, Y., Cui, Y., & Chen, W. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00289 · Cited by 1,769
Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
Zhang, N., Dong, Y., Jia, M., Bian, X., Wang, Y., Qiu, M., Xu, J., Liu, Y., Jiao, L., & Cheng, F. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.8b00565 · Cited by 1,052
Expanded hydrated vanadate for high-performance aqueous zinc-ion batteries
Liu, C., Neale, Z., Zheng, J., Jia, X., Huang, J., Yan, M., Tian, M., Wang, M., Yang, J., & Cao, G. (2019) · Energy & Environmental Science · doi:10.1039/c9ee00956f · Cited by 804
Nam, K. W., Park, S. S., dos Reis, R., Dravid, V. P., Kim, H., Mirkin, C. A., & Stoddart, J. F. (2019) · Nature Communications · doi:10.1038/s41467-019-12857-4 · Cited by 688
Metadata
- Authors
- Xia, C., Guo, J., Li, P., Zhang, X., & Alshareef, H. N.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-02-23
- Volume
- 57
- Issue
- 15
- Pages
- 3943-3948
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2789135099
- Cited by
- 946
- References
- 0
- FWCI
- 44.69
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xia, C., Guo, J., Li, P., Zhang, X., & Alshareef, H. N. (2018). Highly Stable Aqueous Zinc‐Ion Storage Using a Layered Calcium Vanadium Oxide Bronze Cathode. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201713291
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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