The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
An Amorphous Noble‐Metal‐Free Electrocatalyst that Enables Nitrogen Fixation under Ambient Conditions
Abstract
N 2 fixation by the electrocatalytic nitrogen reduction reaction (NRR) under ambient conditions is regarded as a potential approach to achieve NH 3 production, which still heavily relies on the Haber–Bosch process at the cost of huge energy and massive production of CO 2. A noble‐metal‐free Bi 4 V 2 O 11/CeO 2 hybrid with an amorphous phase (BVC‐A) is used as the cathode for electrocatalytic NRR. The amorphous Bi 4 V 2 O 11 contains significant defects, which play a role as active sites. The CeO 2 not only serves as a trigger to induce the amorphous structure, but also establishes band alignment with Bi 4 V 2 O 11 for rapid interfacial charge transfer. Remarkably, BVC‐A shows outstanding electrocatalytic NRR performance with high average yield (NH 3: 23.21 μg h−1 mg−1cat., Faradaic efficiency: 10.16 %) under ambient conditions, which is superior to the Bi 4 V 2 O 11/CeO 2 hybrid with crystalline phase (BVC‐C) counterpart.
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Cites
Combining theory and experiment in electrocatalysis: Insights into materials design
Seh, Z. W., Kibsgaard, J., Dickens, C. F., Chorkendorff, I., Nørskov, J. K., & Jaramillo, T. F. (2017) · Science · doi:10.1126/science.aad4998 · Cited by 12,114
Faber, M. S., & Jin, S. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01760a · Cited by 1,317
Cited by
Efficient Electrocatalytic N2 Fixation with MXene under Ambient Conditions
Luo, Y., Chen, G.-F., Ding, L., Chen, X., Ding, L.-X., & Wang, H. (2019) · Joule · doi:10.1016/j.joule.2018.09.011 · Cited by 699
Self-citationDefect engineering in earth-abundant electrocatalysts for CO2 and N2 reduction
Wang, Q., Lei, Y., Wang, D., & Li, Y. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03781g · Cited by 574
Greatly Improving Electrochemical N 2 Reduction over TiO 2 Nanoparticles by Iron Doping
Wu, T., Zhu, X., Xing, Z., Mou, S., Li, C., Qiao, Y., Liu, Q., Luo, Y., Shi, X., Zhang, Y., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201911153 · Cited by 499
Two-dimensional MXene-based and MXene-derived photocatalysts: Recent developments and perspectives
Zhong, Q., Li, Y., & Zhang, G. (2021) · Chemical Engineering Journal · doi:10.1016/j.cej.2020.128099 · Cited by 466
Han, J., Liu, Z., Ma, Y., Cui, G., Xie, F., Wang, F., Wu, Y., Gao, S., Xu, Y., & Sun, X. (2018) · Nano Energy · doi:10.1016/j.nanoen.2018.07.045 · Cited by 361
Metadata
- Authors
- Lv, C., Yan, C., Chen, G., Ding, Y., Sun, J., Zhou, Y., & Yu, G.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-03-23
- Volume
- 57
- Issue
- 21
- Pages
- 6073-6076
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2792027158
- Cited by
- 664
- References
- 2
- FWCI
- 24.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lv, C., Yan, C., Chen, G., Ding, Y., Sun, J., Zhou, Y., & Yu, G. (2018). An Amorphous Noble‐Metal‐Free Electrocatalyst that Enables Nitrogen Fixation under Ambient Conditions. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201801538
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