The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Ionothermal Synthesis of Triazine–Heptazine‐Based Copolymers with Apparent Quantum Yields of 60 % at 420 nm for Solar Hydrogen Production from “Sea Water”
Abstract
Polymeric carbon nitride (PCN), in either triazine or heptazine form, has been regarded as a promising metal‐free, environmentally benign, and sustainable photocatalyst for solar hydrogen production. However, PCN in most cases only exhibits moderate activity owing to its inherent properties, such as rapid charge carrier recombination. Herein we present a triazine–heptazine copolymer synthesized by simple post‐calcination of PCN in eutectic salts, that is, NaCl/KCl, to modulate the polymerization process and optimize the structure. The construction of an internal triazine–heptazine donor–acceptor (D‐A) heterostructure was affirmed to significantly accelerate interface charge transfer (CT) and thus boost the photocatalytic activity (AQY=60 % at 420 nm). This study highlights the construction of intermolecular D‐A copolymers in NaCl/KCl molten salts with higher melting points but in the absence of lithium to modulate the chemical structure and properties of PCN.
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Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
A Graphitic‐C 3 N 4 “Seaweed” Architecture for Enhanced Hydrogen Evolution
Han, Q., Wang, B., Zhao, Y., Hu, C., & Qu, L. (2015) · Angewandte Chemie International Edition · doi:10.1002/anie.201504985 · Cited by 472
Cited by
Enhanced Photocatalytic H2O2 Production over Carbon Nitride by Doping and Defect Engineering
Wu, S., Yu, H., Chen, S., & Quan, X. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03359 · Cited by 466
Gunawan, D., Zhang, J., Li, Q., Toe, C. Y., Scott, J., Antonietti, M., Guo, J., & Amal, R. (2024) · Advanced Materials · doi:10.1002/adma.202404618 · Cited by 325
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Metadata
- Authors
- Zhang, G., Lin, L., Li, G., Zhang, Y., Savateev, A., Zafeiratos, S., Wang, X., & Antonietti, M.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-06-26
- Volume
- 57
- Issue
- 30
- Pages
- 9372-9376
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2805371382
- Cited by
- 504
- References
- 2
- FWCI
- 13.52
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, G., Lin, L., Li, G., Zhang, Y., Savateev, A., Zafeiratos, S., Wang, X., & Antonietti, M. (2018). Ionothermal Synthesis of Triazine–Heptazine‐Based Copolymers with Apparent Quantum Yields of 60 % at 420 nm for Solar Hydrogen Production from “Sea Water”. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201804702
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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