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Crystalline Covalent Triazine Frameworks by In Situ Oxidation of Alcohols to Aldehyde Monomers
Abstract
Covalent triazine frameworks (CTFs) with aromatic triazine linkages have recently received increasing interest for various applications because of their rich nitrogen content and high chemical stability. Owing to the strong aromatic C=N bond and high chemical stability, only a few CTFs are crystalline, and most CTFs are amorphous. Herein we report a new general strategy to give highly crystalline CTFs by in situ formation of aldehyde monomers through the controlled oxidation of alcohols. This general strategy allows a series of crystalline CTFs with different monomers to be prepared, which are shown to have higher thermal stability and enhanced performance in photocatalysis as compared with the less crystalline or amorphous CTFs. This open‐system approach is very simple and convenient, which presents a potential pathway to large‐scale industrial production of crystalline CTFs.
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Cited by
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
(2021) · doi:10.1038/s41467-021-26817-4 · Cited by 222
Machine Learning‐Assisted Design of Nitrogen‐Rich Covalent Triazine Frameworks Photocatalysts
Wu, M., Song, Z., Cui, Y., Fu, Z., Hong, K., Li, Q., Lyu, Z., Liu, W., & Wang, J. (2025) · Advanced Functional Materials · doi:10.1002/adfm.202413453 · Cited by 17
Wu, M., Sun, J., Cui, Y., Fan, L., Hong, K., Liu, W., Li, Q., Lyu, Z., & Wang, J. (2025) · Advanced Functional Materials · doi:10.1002/adfm.202505234 · Cited by 11
Metadata
- Authors
- Liu, M., Huang, Q., Wang, S., Li, Z., Li, B., Jin, S., & Tan, B.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-08-20
- Volume
- 57
- Issue
- 37
- Pages
- 11968-11972
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2886634470
- Cited by
- 385
- References
- 0
- FWCI
- 12.29
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Liu, M., Huang, Q., Wang, S., Li, Z., Li, B., Jin, S., & Tan, B. (2018). Crystalline Covalent Triazine Frameworks by In Situ Oxidation of Alcohols to Aldehyde Monomers. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201806664
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