The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Salt‐Based Organic–Inorganic Nanocomposites: Towards A Stable Lithium Metal/Li10GeP2S12 Solid Electrolyte Interface
Open accessAbstract
Solid‐state Li metal battery technology is attractive, owing to the high energy density, long lifespans, and better safety. A key obstacle in this technology is the unstable Li/solid‐state electrolyte (SSE) interface involving electrolyte reduction by Li. Herein we report a novel approach based on the use of a nanocomposite consisting of organic elastomeric salts (LiO‐(CH 2 O)n‐Li) and inorganic nanoparticle salts (LiF, ‐NSO 2‐Li, Li 2 O), which serve as an interphase to protect Li 10 GeP 2 S 12 (LGPS), a highly conductive but reducible SSE. The nanocomposite is formed in situ on Li via the electrochemical decomposition of a liquid electrolyte, thus having excellent chemical and electrochemical stability, affinity for Li and LGPS, and limited interfacial resistance. XPS depth profiling and SEM show that the nanocomposite effectively restrained the reduction of LGPS. Stable Li electrodeposition over 3000 h and a 200 cycle life for a full cell were achieved.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Interface Stability in Solid-State Batteries
Richards, W. D., Miara, L. J., Wang, Y., Kim, J. C., & Ceder, G. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b04082 · Cited by 1,652
Cited by
Designing solid-state electrolytes for safe, energy-dense batteries
Zhao, Q., Stalin, S., Zhao, C.-Z., & Archer, L. A. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0165-5 · Cited by 2,372
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes
Cheng, X.-B., Zhao, C.-Z., Yao, Y.-X., Liu, H., & Zhang, Q. (2019) · Chem · doi:10.1016/j.chempr.2018.12.002 · Cited by 874
Artificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
Zhang, Q., Cao, D., Ma, Y., Natan, A., Aurora, P., & Zhu, H. (2019) · Advanced Materials · doi:10.1002/adma.201901131 · Cited by 709
Metadata
- Authors
- Gao, Y., Wang, D., Li, Y. C., Yu, Z., Mallouk, T. E., & Wang, D.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-09-17
- Volume
- 57
- Issue
- 41
- Pages
- 13608-13612
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2885830293
- Cited by
- 179
- References
- 2
- FWCI
- 8.37
- Type
- journal article
- Language
- en
- Open access
- green
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- Gao, Y., Wang, D., Li, Y. C., Yu, Z., Mallouk, T. E., & Wang, D. (2018). Salt‐Based Organic–Inorganic Nanocomposites: Towards A Stable Lithium Metal/Li10GeP2S12 Solid Electrolyte Interface. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201807304
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