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Eosin Y‐Functionalized Conjugated Organic Polymers for Visible‐Light‐Driven CO2 Reduction with H2O to CO with High Efficiency
Abstract
Visible‐light‐driven photoreduction of CO 2 to energy‐rich chemicals in the presence of H 2 O without any sacrifice reagent is of significance, but challenging. Herein, Eosin Y‐functionalized porous polymers (PEosinY‐N, N=1–3), with high surface areas up to 610 m 2 g−1, are reported. They exhibit high activity for the photocatalytic reduction of CO 2 to CO in the presence of gaseous H 2 O, without any photosensitizer or sacrifice reagent, and under visible‐light irradiation. Especially, PEosinY‐1 derived from coupling of Eosin Y with 1,4‐diethynylbenzene shows the best performance for the CO 2 photoreduction, affording CO as the sole carbonaceous product with a production rate of 33 μmol g−1 h−1 and a selectivity of 92 %. This work provides new insight for designing and fabricating photocatalytically active polymers with high efficiency for solar‐energy conversion.
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In situ click chemistry generation of cyclooxygenase-2 inhibitors
Bhardwaj, A., Kaur, J., Wuest, M., & Wuest, F. (2017) · Nature Communications · doi:10.1038/s41467-016-0009-6 · Cited by 7,448
Cited by
Emerging trends in porous materials for CO2capture and conversion
Singh, G., Lee, J., Karakoti, A., Bahadur, R., Yi, J., Zhao, D., AlBahily, K., & Vinu, A. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00075b · Cited by 843
Conjugated polymers for visible-light-driven photocatalysis
Dai, C., & Liu, B. (2020) · Energy & Environmental Science · doi:10.1039/c9ee01935a · Cited by 687
Metadata
- Authors
- Yu, X., Yang, Z., Qiu, B., Guo, S., Yang, P., Yu, B., Zhang, H., Zhao, Y., Yang, X., Han, B., & Liu, Z.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2018-12-12
- Volume
- 58
- Issue
- 2
- Pages
- 632-636
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2903719108
- Cited by
- 223
- References
- 1
- FWCI
- 4.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Yu, X., Yang, Z., Qiu, B., Guo, S., Yang, P., Yu, B., Zhang, H., Zhao, Y., Yang, X., Han, B., & Liu, Z. (2019). Eosin Y‐Functionalized Conjugated Organic Polymers for Visible‐Light‐Driven CO2 Reduction with H2O to CO with High Efficiency. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201812790
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