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Synergy between Plasmonic and Electrocatalytic Activation of Methanol Oxidation on Palladium–Silver Alloy Nanotubes
Abstract
Localized surface plasmon resonance (LSPR) excitation of noble metal nanoparticles has been shown to accelerate and drive photochemical reactions. Here, LSPR excitation is shown to enhance the electrocatalysis of a fuel‐cell‐relevant reaction. The electrocatalyst consists of PdxAg alloy nanotubes (NTs), which combine the catalytic activity of Pd toward the methanol oxidation reaction (MOR) and the visible‐light plasmonic response of Ag. The alloy electrocatalyst exhibits enhanced MOR activity under LSPR excitation with significantly higher current densities and a shift to more positive potentials. The modulation of MOR activity is ascribed primarily to hot holes generated by LSPR excitation of the PdxAg NTs.
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Cited by
Heterogeneous‐Interface‐Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation
Zhou, P., Lv, X., Tao, S., Wu, J., Wang, H., Wei, X., Wang, T., Zhou, B., Lu, Y., Frauenheim, T., et al. (2022) · Advanced Materials · doi:10.1002/adma.202204089 · Cited by 570
High-entropy alloys in electrocatalysis: from fundamentals to applications
Ren, J.-T., Chen, L., Wang, H.-Y., & Yuan, Z.-Y. (2023) · Chemical Society Reviews · doi:10.1039/d3cs00557g · Cited by 551
Recent Progress on Rational Design of Bimetallic Pd Based Catalysts and Their Advanced Catalysis
Fan, J., Du, H., Zhao, Y., Wang, Q., Liu, Y., Li, D., & Feng, J. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c03280 · Cited by 265
Highly Loaded Independent Pt0 Atoms on Graphdiyne for pH‐General Methanol Oxidation Reaction
Hui, L., Xue, Y., Xing, C., Liu, Y., Du, Y., Fang, Y., Yu, H., Huang, B., & Li, Y. (2022) · Advanced Science · doi:10.1002/advs.202104991 · Cited by 57
Halogen Tailoring of Platinum Electrocatalyst with High CO Tolerance for Methanol Oxidation Reaction
Hui, L., Yan, D., Zhang, X., Wu, H., Li, J., & Li, Y. (2024) · Angewandte Chemie International Edition · doi:10.1002/anie.202410413 · Cited by 56
Metadata
- Authors
- Huang, L., Zou, J., Ye, J., Zhou, Z., Lin, Z., Kang, X., Jain, P. K., & Chen, S.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-22
- Volume
- 58
- Issue
- 26
- Pages
- 8794-8798
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2942586823
- Cited by
- 169
- References
- 0
- FWCI
- 4.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, L., Zou, J., Ye, J., Zhou, Z., Lin, Z., Kang, X., Jain, P. K., & Chen, S. (2019). Synergy between Plasmonic and Electrocatalytic Activation of Methanol Oxidation on Palladium–Silver Alloy Nanotubes. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201903290
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