The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Nitriding‐Interface‐Regulated Lithium Plating Enables Flame‐Retardant Electrolytes for High‐Voltage Lithium Metal Batteries
Abstract
Safety concerns are impeding the applications of lithium metal batteries. Flame‐retardant electrolytes, such as organic phosphates electrolytes (OPEs), could intrinsically eliminate fire hazards and improve battery safety. However, OPEs show poor compatibility with Li metal though the exact reason has yet to be identified. Here, the lithium plating process in OPEs and Li/OPEs interface chemistry were investigated through ex situ and in situ techniques, and the cause for this incompatibility was revealed to be the highly resistive and inhomogeneous interfaces. Further, a nitriding interface strategy was proposed to ameliorate this issue and a Li metal anode with an improved Li cycling stability (300 h) and dendrite‐free morphology is achieved. Meanwhile, the full batteries coupled with nickel‐rich cathodes, such as LiNi 0.8 Co 0.1 Mn 0.1 O 2, show excellent cycling stability and outstanding safety (passed the nail penetration test). This successful nitriding‐interface strategy paves a new way to handle the incompatibility between electrode and electrolyte.
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Citations
Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Cited by
Insights into the deposition chemistry of Li ions in nonaqueous electrolyte for stable Li anodes
Wang, Z., Sun, Z., Li, J., Shi, Y., Sun, C., An, B., Cheng, H.-M., & Li, F. (2021) · Chemical Society Reviews · doi:10.1039/d0cs01017k · Cited by 268
Self-citationHan, Y., Liu, B., Xiao, Z., Zhang, W., Wang, X., Pan, G., Xia, Y., Xia, X., & Tu, J. (2021) · InfoMat · doi:10.1002/inf2.12166 · Cited by 267
Wang, Z., Sun, Z., Shi, Y., Qi, F., Gao, X., Yang, H., Cheng, H., & Li, F. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202100935 · Cited by 202
Metadata
- Authors
- Tan, S., Yue, J., Hu, X., Shen, Z., Wang, W., Li, J., Zuo, T., Duan, H., Xiao, Y., Yin, Y., Wen, R., & Guo, Y.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-05-06
- Volume
- 58
- Issue
- 23
- Pages
- 7802-7807
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2937650145
- Cited by
- 202
- References
- 2
- FWCI
- 11.28
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tan, S., Yue, J., Hu, X., Shen, Z., Wang, W., Li, J., Zuo, T., Duan, H., Xiao, Y., Yin, Y., Wen, R., & Guo, Y. (2019). Nitriding‐Interface‐Regulated Lithium Plating Enables Flame‐Retardant Electrolytes for High‐Voltage Lithium Metal Batteries. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201903466
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