The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Encapsulating Perovskite Quantum Dots in Iron‐Based Metal–Organic Frameworks (MOFs) for Efficient Photocatalytic CO2 Reduction
Abstract
Improving the stability of lead halide perovskite quantum dots (QDs) in a system containing water is the key for their practical application in artificial photosynthesis. Herein, we encapsulate low‐cost CH 3 NH 3 PbI 3 (MAPbI 3) perovskite QDs in the pores of earth‐abundant Fe‐porphyrin based metal organic framework (MOF) PCN‐221(Fex) by a sequential deposition route, to construct a series of composite photocatalysts of MAPbI 3@PCN‐221(Fex) (x=0–1). Protected by the MOF the composite photocatalysts exhibit much improved stability in reaction systems containing water. The close contact of QDs to the Fe catalytic site in the MOF, allows the photogenerated electrons in the QDs to transfer rapidly the Fe catalytic sites to enhance the photocatalytic activity for CO 2 reduction. Using water as an electron source, MAPbI 3@PCN‐221(Fe 0.2) exhibits a record‐high total yield of 1559 μmol g−1 for photocatalytic CO 2 reduction to CO (34 %) and CH 4 (66 %), 38 times higher than that of PCN‐221(Fe 0.2) in the absence of perovskite QDs.
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Citations
Cites
Genesis, challenges and opportunities for colloidal lead halide perovskite nanocrystals
Akkerman, Q. A., Rainò, G., Kovalenko, M. V., & Manna, L. (2018) · Nature Materials · doi:10.1038/s41563-018-0018-4 · Cited by 2,287
Cited by
Sheng, J., He, Y., Li, J., Yuan, C., Huang, H., Wang, S., Sun, Y., Wang, Z., & Dong, F. (2020) · ACS Nano · doi:10.1021/acsnano.0c04659 · Cited by 522
Younas, M., Rezakazemi, M., Daud, M., Wazir, M. B., Ahmad, S., Ullah, N., Inamuddin, & Ramakrishna, S. (2020) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2020.100849 · Cited by 421
Jiang, Y., Liao, J.-F., Chen, H.-Y., Zhang, H.-H., Li, J.-Y., Wang, X.-D., & Kuang, D.-B. (2020) · Chem · doi:10.1016/j.chempr.2020.01.005 · Cited by 404
Dai, Y., Poidevin, C., Ochoa‐Hernández, C., Auer, A. A., & Tüysüz, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201915034 · Cited by 269
Application of aluminosilicate clay mineral-based composites in photocatalysis
Zou, Y., Hu, Y., Shen, Z., Yao, L., Tang, D., Zhang, S., Wang, S., Hu, B., Zhao, G., & Wang, X. (2022) · Journal of Environmental Sciences · doi:10.1016/j.jes.2021.07.015 · Cited by 117
Metadata
- Authors
- Wu, L., Mu, Y., Guo, X., Zhang, W., Zhang, Z., Zhang, M., & Lu, T.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-06-06
- Volume
- 58
- Issue
- 28
- Pages
- 9491-9495
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2944125431
- Cited by
- 776
- References
- 1
- FWCI
- 19.07
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wu, L., Mu, Y., Guo, X., Zhang, W., Zhang, Z., Zhang, M., & Lu, T. (2019). Encapsulating Perovskite Quantum Dots in Iron‐Based Metal–Organic Frameworks (MOFs) for Efficient Photocatalytic CO2 Reduction. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201904537
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