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Redox‐Active Two‐Dimensional Covalent Organic Frameworks (COFs) for Selective Reductive Separation of Valence‐Variable, Redox‐Sensitive and Long‐Lived Radionuclides
Abstract
We report the first example of 2D covalent organic framework nanosheets (Redox‐COF1) for the selective reduction and in situ loading of valence‐variable, redox‐sensitive and long‐lived radionuclides (abbreviated as VRL nuclides). Compared with sorbents based on chemical adsorption and physical adsorption, the redox adsorption mechanism of Redox‐COF1 can effectively reduce the impact of functional group protonation under the usual high‐acidity conditions in chemisorption, and raise the adsorption efficiency from the monotonous capture by pores in physisorption. The adsorption selectivity for UO 22+ reaches up to unprecedented ca. 97 % at pH 3, more than for any analogous adsorbing material.
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Paiva, A. P., & Malik, P. (2004) · Journal of Radioanalytical and Nuclear Chemistry · doi:10.1023/b:jrnc.0000034890.23325.b5 · Cited by 290
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Chen, Z., He, X., Li, Q., Yang, H., Liu, Y., Wu, L., Liu, Z., Hu, B., & Wang, X. (2022) · Journal of Environmental Sciences · doi:10.1016/j.jes.2021.10.003 · Cited by 56
Metadata
- Authors
- Li, Y., Guo, X., Li, X., Zhang, M., Jia, Z., Deng, Y., Tian, Y., Li, S., & Ma, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2020-01-22
- Volume
- 59
- Issue
- 10
- Pages
- 4168-4175
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2994870326
- Cited by
- 191
- References
- 1
- FWCI
- 7.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Redox‐Active Two‐Dimensional Covalent Organic Frameworks (COFs) for Selective Reductive Separation of Valence‐Variable, Redox‐Sensitive and Long‐Lived Radionuclides. https://app.cochat.ai/papers/10.1002/anie.201916360
- The paper
- Li, Y., Guo, X., Li, X., Zhang, M., Jia, Z., Deng, Y., Tian, Y., Li, S., & Ma, L. (2020). Redox‐Active Two‐Dimensional Covalent Organic Frameworks (COFs) for Selective Reductive Separation of Valence‐Variable, Redox‐Sensitive and Long‐Lived Radionuclides. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201916360
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